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Record W2008303678 · doi:10.1002/3527605487.ch7

Polyynes Via Alkylidene Carbenes and Carbenoids

2004· other· en· W2008303678 on OpenAlexafffund
Sara Eisler, Rik R. Tykwinski

Bibliographic record

Venuenot available
Typeother
Languageen
FieldChemistry
TopicCyclopropane Reaction Mechanisms
Canadian institutionsUniversity of Alberta
FundersNatural Sciences and Engineering Research Council of Canada
KeywordsCarbenoidCarbeneConjugated systemChemistryAcylationCombinatorial chemistryAlkyneStereochemistryOrganic chemistryCatalysisRhodium

Abstract

fetched live from OpenAlex

This chapter contains sections titled: Introduction Alkylidene Carbene and Carbenoid Species Alkyne Formation from Carbenes and Carbenoids Synthesis of Acetylenes: the Fritsch–Buttenberg–Wiechell Rearrangement Synthesis of 1,3–Butadiynes Synthesis of 1,3,5–Hexatriynes Tri- and Pentaynes from Free Alkylidene Carbenes Toward applications Natural Products Synthesis Extended Arylenethynylene Derivatives Cyclo[n]carbons Linear Conjugated Polyynes Synthesis of Triisopropylsilyl End-Capped Polyynes Solid-State Characterization Linear Optical Properties Third-Order Nonlinear Optical Properties Conclusions Experimental Procedures General Procedure for Friedel–Crafts Acylation General Procedure for Dibromoolefination General FBW Rearrangement Procedure General Oxidative Coupling Procedure Acknowledgements

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow), Insufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: none
GenreCandidate signal: Other · Consensus signal: Other
Teacher disagreement score0.688
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0010.000
Insufficient payload (model declined to judge)0.0200.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.005
GPT teacher head0.209
Teacher spread0.204 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreOther

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations6
Published2004
Admission routes2
Has abstractyes

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