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Record W2012949478 · doi:10.1149/05313.0001ecst

A Quantitative Study of Hydroxyl Radical Production on a Ti/SnO<sub>2</sub>-Sb<sub>2</sub>O<sub>5</sub> Anode

2013· article· en· W2012949478 on OpenAlex
Qing Ni, Donald W. Kirk, Steven J. Thorpe

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.

Bibliographic record

VenueECS Transactions · 2013
Typearticle
Languageen
FieldChemistry
TopicPigment Synthesis and Properties
Canadian institutionsUniversity of Toronto
Fundersnot available
KeywordsElectrolysisAnodeAnalytical Chemistry (journal)Oxygen evolutionElectrodeRadicalElectrolyteStoichiometryChemistryHydroxyl radicalMaterials scienceInorganic chemistryElectrochemistryPhysical chemistryOrganic chemistry

Abstract

fetched live from OpenAlex

A nitroso compound (R-NO) known as a “spin trap” was used to study the production of hydroxyl radicals (OH·) on a Ti/SnO 2 -Sb 2 O 5 anode. A linear voltammetry study was conducted on this anode in the presence of this compound, using the rotating disk electrode technique. The results showed that the electrode started to produce (OH·) at 0.7V vs. Ag/AgCl reference electrode. The current was limited by the mass-transport of RNO in the electrolyte. When the voltage increased to 1.4V and higher, significant oxygen evolution took place. Further investigation was conducted by constant voltage electrolysis and spectroscopic measurement of the RNO concentration. The change in the RNO was interpreted as the evolution of (OH·), and the current efficiency was calculated based on the assumed stoichiometry. The results showed that the efficiency was optimal within the potential range 0.7-1.4V, and the highest efficiency could reach 30%. This was in agreement with the RDE experiment.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.016
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0010.001
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.001
Science and technology studies0.0010.000
Scholarly communication0.0000.001
Open science0.0000.000
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0000.001

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.023
GPT teacher head0.233
Teacher spread0.210 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it