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Record W2013370730 · doi:10.1063/1.1406499

Large enhancement in dissociative electron attachment to HCl adsorbed on H2O ice via transfer of presolvated electrons

2001· article· en· W2013370730 on OpenAlexaff
Qing‐Bin Lu, Léon Sanche

Bibliographic record

VenueThe Journal of Chemical Physics · 2001
Typearticle
Languageen
FieldEarth and Planetary Sciences
TopicAtmospheric Ozone and Climate
Canadian institutionsCanadian Institutes of Health ResearchUniversité de Sherbrooke
Fundersnot available
KeywordsDissociation (chemistry)AdsorptionElectronIonizationElectron transferChemistryElectron ionizationSolvated electronElectron captureAtomic physicsPolarChemical physicsPhotochemistryIonPhysical chemistryPhysicsRadiolysisOrganic chemistry

Abstract

fetched live from OpenAlex

We report that dissociative electron attachment (DEA) to HCl is strongly enhanced by adsorption on the surface of H2O ice. The absolute DEA cross section at ∼0 eV for HCl adsorbed on ice is measured to be ∼4.0×10−15 cm2, which is two orders of magnitude higher than in the gas phase. This enhancement is essentially due to electron transfer from precursor states of the solvated electron in ice to an unfilled molecular orbital of HCl followed by its dissociation. This study indicates that electron-induced dissociation may be a significant process leading to HCl dissociation on ice surfaces in polar stratospheric clouds due to ionization by cosmic rays.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.051
Threshold uncertainty score0.298

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.009
GPT teacher head0.245
Teacher spread0.237 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations49
Published2001
Admission routes1
Has abstractyes

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