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Record W2014507633 · doi:10.1021/ef1015704

Simultaneous Adsorption of H<sub>2</sub>S and CO<sub>2</sub> on Triamine-Grafted Pore-Expanded Mesoporous MCM-41 Silica

2011· article· en· W2014507633 on OpenAlex
Youssef Belmabkhout, Nicolas Heymans, Guy De Weireld, Abdelhamid Sayari

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.

Bibliographic record

VenueEnergy & Fuels · 2011
Typearticle
Languageen
FieldEngineering
TopicCarbon Dioxide Capture Technologies
Canadian institutionsUniversity of Ottawa
Fundersnot available
KeywordsAdsorptionMesoporous materialMCM-41Amine gas treatingMesoporous silicaChemistryChemical engineeringNuclear chemistryMolecular sieveOrganic chemistryCatalysis

Abstract

fetched live from OpenAlex

The feasibility of using triamine-grafted pore-expanded mesoporous MCM-41 silica (TRI-PE-MCM-41) as a potential adsorbent for simultaneous removal of CO 2 and H 2 S was investigated. Adsorption isotherms of CO 2 and H 2 S were measured at different temperatures, whereas adsorption at low H 2 S concentrations from 700 to 10000 ppm with balance CO 2 was studied at 298 K. It was found that both CO 2 and H 2 S adsorb and the selectively toward H 2 S versus CO 2 decreases at an increasing H 2 S concentration. Because TRI-PE-MCM-41 hardly adsorbs any of the common gases, such as CH 4, H 2, N 2, O 2, and CO, it was inferred that this material may be suitable for the purification of a variety of gas streams containing CO 2 and H 2 S. These findings lay the ground for the development of a single-stage process for the removal of CO 2 and H 2 S from biogas, using amine-supported PE-MCM-41.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.028
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0010.001
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0010.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.011
GPT teacher head0.199
Teacher spread0.188 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it