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Record W2020539038 · doi:10.3139/217.1017

Dynamically Vulcanized Nanocomposite Thermoplastic Elastomers Based on EPDM/PP (Rheology & Morphology)

2007· article· en· W2020539038 on OpenAlex
Ghasem Naderi, Pierre G. Lafleur, Charles Dubois

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.

Bibliographic record

VenueInternational Polymer Processing · 2007
Typearticle
Languageen
FieldMaterials Science
TopicPolymer Nanocomposites and Properties
Canadian institutionsPolytechnique Montréal
Fundersnot available
KeywordsMaterials scienceVulcanizationComposite materialRheometryNanocompositePolypropyleneNatural rubberThermoplastic elastomerRheologyViscoelasticityElastomerPolymerCopolymer

Abstract

fetched live from OpenAlex

Abstract This study examines the rheological and morphological properties of dynamically vulcanized nanocomposite thermoplastic elastomers (TPV nanocomposites) based on PP/EPDM. Rubber contents of 20, 40, and 60% were used with polypropylene of different viscosities at 2 wt.% of nanoclay. We performed rheological and morphological characterizations on the nanocomposites using X-ray diffraction, transmission electron microscopy, scanning electron microscopy and rheometry in small amplitude oscillatory shear. The effects of polypropylene viscosity, maleic anhydride grafted polypropylene (PPMA), and composition were also investigated. The storage modulus (G) of the TPV nanocomposites (without PPMA) containing 20, 40, and 60% rubber significantly increased in comparison with similar but unfilled samples and also a further increase in the G from the incorporation of the PPMA in the samples. The agglomeration of the clay considerably decreased when the rubber content was increased in the TPV nanocomposites. The yield stress of the prepared TPV nanocomposite, based on a low-viscosity PP, increased more than that of the sample from high viscosity PP. The TPV nanocomposites containing 20, 40 and 60% EPDM exhibited a strong elastic modulus that tended to level off (plateau) at low shear rates. These results were attributed to strong interfacial interactions between the nanoclay and TPV matrix and, also, the existence of the physical three-dimensional network structure formed between the cured rubber particles, as evidenced by the morphological features of the samples. A Carreau-Yasuda law with yield stress and a linear viscoelastic model, taking into account the maximum packing volume () were used to describe the melt linear viscoelastic properties of the TPV nanocomposites.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow), Insufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.050
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0010.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.001

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.011
GPT teacher head0.261
Teacher spread0.250 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it