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Record W2021567446 · doi:10.1103/physreva.73.013412

Molecules in intense laser fields: Beyond the dipole approximation

2006· article· en· W2021567446 on OpenAlexaff
André D. Bandrauk, Huizhong Lu

Bibliographic record

VenuePhysical Review A · 2006
Typearticle
Languageen
FieldPhysics and Astronomy
TopicLaser-Matter Interactions and Applications
Canadian institutionsUniversité de Sherbrooke
Fundersnot available
KeywordsPhysicsAtomic physicsDipoleElectronElectric fieldHarmonicsWavelengthPolarization (electrochemistry)LambdaSpectral linePhoton energyPhotonQuantum mechanicsVoltage

Abstract

fetched live from OpenAlex

The time-dependent Schr\"odinger equation is solved for a Born-Oppenheimer (static nuclei) three-dimensional $\mathrm{H}_{2}{}^{+}$ in super intense laser fields ($I=4\ifmmode\times\else\texttimes\fi{}{10}^{18}$, ${10}^{19}$, and $4\ifmmode\times\else\texttimes\fi{}{10}^{19}\phantom{\rule{0.3em}{0ex}}\mathrm{W}∕{\mathrm{cm}}^{2}$) at wavelength ${\ensuremath{\lambda}}_{L}=45\phantom{\rule{0.3em}{0ex}}\mathrm{nm}$ and $25\phantom{\rule{0.3em}{0ex}}\mathrm{nm}$ to assess the influence of nondipolar (magnetic) effects on high order harmonic generation spectra in molecules. It is found that even harmonics appear due to the magnetic field component direction perpendicular to the electric field polarization with intensities about two orders of magnitude less than the odd harmonics emitted along the electric field polarization. The even harmonics exhibit plateaus with cutoffs which exceed in intensity the odd harmonic plateaus and maximum energies predicted by semiclassical electron recollision models. Although the spectra are weak, the wavelength of the recollision electron in the maximum energy regions correspond to subatomic dimensions and the corresponding emitted photons have subnanometer wavelengths.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Theoretical or conceptual · Consensus signal: Theoretical or conceptual
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.207
Threshold uncertainty score0.373

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.008
GPT teacher head0.282
Teacher spread0.274 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designTheoretical or conceptual
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations23
Published2006
Admission routes1
Has abstractyes

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Same venuePhysical Review ASame topicLaser-Matter Interactions and ApplicationsFrench-language works237,207