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Record W2021854219 · doi:10.1080/17415993.2010.527981

Ethylene manufacture by partial oxidation with sulfur

2010· article· en· W2021854219 on OpenAlexafffund
Peter D. Clark, Norman I. Dowling, S. Liu

Bibliographic record

VenueJournal of Sulfur Chemistry · 2010
Typearticle
Languageen
FieldEngineering
TopicCatalysis and Hydrodesulfurization Studies
Canadian institutionsUniversity of Calgary
FundersUniversity of Calgary
KeywordsEthyleneSulfurChemistryYield (engineering)CrackingSour gasClaus processCarbon fibersOrganic chemistryInorganic chemistryCatalysisMetallurgyMaterials scienceNatural gasHydrogen sulfide

Abstract

fetched live from OpenAlex

The objective of this study was to examine the sulfur-mediated oxidation of ethane to ethylene. In summary, it has been found that ethylene can be produced in high yield (ca 75%) by the oxidation of ethane with excess sulfur in the 800–850 °C temperature range using a residence time of about 1 s. It is surmised that the high ethylene yield arises from the relatively weak C–S bond which precludes the formation of carbon–sulfur compounds so favoring pathways to ethylene. A process scheme is suggested which incorporates ethylene production into sulfur recovery, plants for which are found in essentially all refineries and in sour gas processing. A potential advantage of this chemistry over standard ethane steam cracking is that the sulfur process considerably increases carbon efficiency for ethylene production as most of the energy required for ethylene synthesis is supplied by the oxidation of H2S.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.022
Threshold uncertainty score0.485

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.003
GPT teacher head0.187
Teacher spread0.184 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations3
Published2010
Admission routes2
Has abstractyes

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