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Record W2031458076 · doi:10.1021/ie0499153

Selective Rejection of Inorganic Fine Solids, Heavy Metals, and Sulfur from Heavy Oils/Bitumen Using Alkane Solvents

2004· article· en· W2031458076 on OpenAlexafffund
Xiang-Yang Zou, Leisl Dukhedin-Lalla, Xiaohui Zhang, John M. Shaw

Bibliographic record

VenueIndustrial & Engineering Chemistry Research · 2004
Typearticle
Languageen
FieldChemistry
TopicPetroleum Processing and Analysis
Canadian institutionsUniversity of Alberta
FundersNatural Sciences and Engineering Research Council of CanadaUniversity of TorontoUniversity of AlbertaGovernment of Ontario
KeywordsAlkanePentaneDodecaneChemistryDecaneHeptaneSolventPhase (matter)SulfurHydrocarbonVanadiumInorganic chemistryOrganic chemistry

Abstract

fetched live from OpenAlex

Bitumen and heavy oil + alkane solvents exhibit complex phase behaviors. For example, organic components of these materials can be solubilized and inorganic solids dispersed into a high-pressure gas phase. Conversely, they can also be partitioned into as many as three bulk phases: a gas phase, a liquid phase that is largely free of inorganic solids, and a phase comprising essentially all of the inorganic solids and a small fraction of the organic material. The outcome depends on the temperature, pressure, and solvent-to-feed ratio. Mass balance results for a screening survey for Athabasca vacuum bottoms (ABVB) + alkane solvents (pentane, heptane, decane, and dodecane) are reported along with a limited number of phase composition data for ABVB + pentane and dodecane mixtures. Reversible phase behavior and irreversible thermolysis conditions were considered. The key findings are that inorganic solids are readily partitioned from ABVB irrespective of the solvent and operating conditions employed, while key heavy metals, such as vanadium, require a combination of phase behavior and mild thermolysis. Sulfur- and nitrogen-containing species possess low rejection selectivities in this solvent series.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.003

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.057
GPT teacher head0.306
Teacher spread0.249 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations17
Published2004
Admission routes2
Has abstractyes

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