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Record W2034590105 · doi:10.1002/cjce.22047

On the analysis of ionic mass transfer in the electrolytic bath of an aluminum reduction cell

2014· article· en· W2034590105 on OpenAlexafffundvenue
Mohsen Ariana, Martin Désilets, Pierre Proulx

Bibliographic record

VenueThe Canadian Journal of Chemical Engineering · 2014
Typearticle
Languageen
FieldMaterials Science
TopicAnodic Oxide Films and Nanostructures
Canadian institutionsUniversité de Sherbrooke
FundersNatural Sciences and Engineering Research Council of Canada
KeywordsElectrolyteElectrolysisIonElectrochemistryChemistryDiffusionIonic bondingMass transferElectric fieldElectrodeCurrent densityDiffusion currentAnalytical Chemistry (journal)Electrolytic cellChemical physicsInorganic chemistryThermodynamicsCurrent (fluid)Physical chemistryChromatography

Abstract

fetched live from OpenAlex

Abstract An electrolyte typically used in an aluminum electrolysis cell is composed of different ions moving in the electromagnetic field generated by the high intensity current needed for the industrial application. The flux of these ions has an important impact on the functional parameters of the cell, like current efficiency. In this study, the transient behaviour of these ions in the NaF‐AlF3‐Al2O3 mixture is modelled using a numerical finite element method. The electric potential field equation governed by electrochemical reaction kinetics at electrodes is solved to obtain the electric potential field, current density, and consequently heat generation in the cell. Subsequently, the concentration field is solved for ionic species in the bath. The results indicate formation of a high concentration gradient of electroactive ions like Al2OF62− and AlF4− at the corresponding reacting electrodes with time and diffusion as the main mechanism for these ions transfer. It is found that from the early stages of the 3 minute simulation of the electrochemical process, the difference between bulk concentration and surface concentration of electroactive ions remains constant. Moreover, the results indicate that although the flux of electroactive species is dominated by diffusion, especially for larger times, migration is the controlling mechanism of transport for the electroinactive ions.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.004
Threshold uncertainty score0.008

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0010.000
Insufficient payload (model declined to judge)0.0020.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.004
GPT teacher head0.172
Teacher spread0.168 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations16
Published2014
Admission routes3
Has abstractyes

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Same venueThe Canadian Journal of Chemical EngineeringSame topicAnodic Oxide Films and NanostructuresFrench-language works237,207