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Record W2034590105 · doi:10.1002/cjce.22047

On the analysis of ionic mass transfer in the electrolytic bath of an aluminum reduction cell

2014· article· en· W2034590105 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.
fundA Canadian funder is recorded on the work.
venuePublished in a venue whose home country is Canada.

Bibliographic record

VenueThe Canadian Journal of Chemical Engineering · 2014
Typearticle
Languageen
FieldMaterials Science
TopicAnodic Oxide Films and Nanostructures
Canadian institutionsUniversité de Sherbrooke
FundersNatural Sciences and Engineering Research Council of Canada
KeywordsElectrolyteElectrolysisIonElectrochemistryChemistryDiffusionIonic bondingMass transferElectric fieldElectrodeCurrent densityDiffusion currentAnalytical Chemistry (journal)Electrolytic cellChemical physicsInorganic chemistryThermodynamicsCurrent (fluid)Physical chemistryChromatography

Abstract

fetched live from OpenAlex

Abstract An electrolyte typically used in an aluminum electrolysis cell is composed of different ions moving in the electromagnetic field generated by the high intensity current needed for the industrial application. The flux of these ions has an important impact on the functional parameters of the cell, like current efficiency. In this study, the transient behaviour of these ions in the NaF‐AlF 3 ‐Al 2 O 3 mixture is modelled using a numerical finite element method. The electric potential field equation governed by electrochemical reaction kinetics at electrodes is solved to obtain the electric potential field, current density, and consequently heat generation in the cell. Subsequently, the concentration field is solved for ionic species in the bath. The results indicate formation of a high concentration gradient of electroactive ions like Al 2 OF 6 2− and AlF 4 − at the corresponding reacting electrodes with time and diffusion as the main mechanism for these ions transfer. It is found that from the early stages of the 3 minute simulation of the electrochemical process, the difference between bulk concentration and surface concentration of electroactive ions remains constant. Moreover, the results indicate that although the flux of electroactive species is dominated by diffusion, especially for larger times, migration is the controlling mechanism of transport for the electroinactive ions.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.018
Threshold uncertainty score0.141

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.004
GPT teacher head0.172
Teacher spread0.168 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it