MétaCan
Menu
← all works

Reaction of Li with Alloy Thin Films Studied by In Situ AFM

2003· article· en· 622 citations· W2035395460 on OpenAlex· 10.1149/1.1613668

Why is this work in the frame?

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

Canadian affiliationAn author listed a Canadian institution. This is the only route the usual frame has.

Full frame distilled prediction

Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

Candidate categories
none
Consensus categories
none
Domain
Candidate signal: noneConsensus signal: none
Study design
Candidate signal: Bench or experimentalConsensus signal: Bench or experimental
Genre
Candidate signal: EmpiricalConsensus signal: Empirical
Teacher disagreement score
0.004
Threshold uncertainty score
0.257
Validation status
machine_predicted_unvalidated · codex-gemma-dda1882f352a

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Opus teacher head0.006
GPT teacher head0.219
Teacher spread
0.213 · how far apart the two teachers sit on this one work
Validation status
score_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Abstract

Many intermetallic materials deliver poor capacity retention when cycled vs. Li. Many authors have attributed this poor capacity retention to large volume expansions of the active material. Here we report the volume changes of continuous and patterned films of crystalline Al, crystalline Sn, amorphous Si (a-Si), and as they reversibly react with Li measured by in situ atomic force microscopy (AFM). Although these materials all undergo large volume expansions, the amorphous phases undergo reversible shape and volume changes. The crystalline materials do not. We attribute this difference to the homogeneous expansion and contraction that occurs in the amorphous materials. Inhomogeneous expansion occurs in the crystalline materials due to the presence of coexisting phases with different Li concentrations. Thin films of a-Si and show good capacity retention with cycle number. © 2003 The Electrochemical Society. All rights reserved.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

The record

Venue
Journal of The Electrochemical Society
Topic
Advancements in Battery Materials
Field
Engineering
Canadian institutions
Dalhousie University
Funders
not available
Keywords
Amorphous solidMaterials scienceIntermetallicIn situAlloyHomogeneousAtomic force microscopyChemical engineeringVolume (thermodynamics)Thin filmElectrochemistryComposite materialNanotechnologyCrystallographyElectrodeChemistryThermodynamicsPhysical chemistryOrganic chemistry
Has abstract in OpenAlex
yes