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Long-Lived Transient Vacancy Distribution in Multilayers

2005· article· en· W2037877497 on OpenAlexaff
Jean-Marc Roussel, Pascal Bellon

Bibliographic record

VenueDefect and diffusion forum/Diffusion and defect data, solid state data. Part A, Defect and diffusion forum · 2005
Typearticle
Languageen
FieldEarth and Planetary Sciences
Topicnanoparticles nucleation surface interactions
Canadian institutionsCegep de Saint Jerome
Fundersnot available
KeywordsVacancy defectKinetic Monte CarloCondensed matter physicsKinetic energyPhase (matter)DiffusionMaterials scienceLattice (music)Ising modelMonte Carlo methodThermodynamicsChemistryPhysics

Abstract

fetched live from OpenAlex

Modeling the vacancy concentration in bi-metallic systems is a key step to understand thermal interdiffusion phenomena. For instance in the kinetics of precipitation, a strong difference between vacancy concentration in the precipitates and in the matrix, may change the precipitate mobility and the coarsening mechanism, the precipitate composition and morphology [1]. The origin of this inhomogeneous vacancy concentration is mainly due to the differences in migration energies ∆E and in formation energies ∆E of the vacancy in the two phases. The distribution of vacancy sinks and sources or the local lattice deformation should also play an important role. In this work, we focus on the influence of both ∆E and ∆E terms on the vacancy concentration profile in a phase separating a multilayer with planar (111) interfaces. The atomic diffusion model is a kinetic Ising-like model with a vacancy exchange mechanism. We perform both kinetic Mean-field and kinetic Monte-Carlo simulations in order to discuss how the vacancy concentration profile (VCP) reaches its steady-state. In the figure, we report the quasistationary VCP found at the vicinity of an (111) interface for ∆E = 0eV. As expected the vacancy strongly segregates into the two interface planes (p=-1,0) because of the tendency of the system to phase separate (the vacancy tends to reduce the number of AB pairs). More surprising is the decrease of the concentration in adjacent planes (p=-3,2,1,2). This marked decrease, that becomes asymmetric for ∆E = -0.1eV (see figure), is rationalized by invoking local correlation effects.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow), Science and technology studies, Insufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Observational · Consensus signal: Observational
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.252
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0010.001
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0010.001
Science and technology studies0.0010.000
Scholarly communication0.0010.002
Open science0.0010.001
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.029
GPT teacher head0.283
Teacher spread0.254 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designObservational
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2005
Admission routes1
Has abstractyes

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