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Record W2039154042 · doi:10.1039/b102979g

Compaction of grafted wormlike chains under variable confinement

2001· article· en· W2039154042 on OpenAlexaff
Gustavo A. Arteca, Tomas Edvinsson, Christer Elvingson

Bibliographic record

VenuePhysical Chemistry Chemical Physics · 2001
Typearticle
Languageen
FieldMaterials Science
TopicPolymer Surface Interaction Studies
Canadian institutionsLaurentian University
Fundersnot available
KeywordsCompactionScalingSlabVariable (mathematics)Persistence lengthChain (unit)Statistical physicsMaterials sciencePolymerChemical physicsPhysicsMathematicsGeometryComposite materialMathematical analysis

Abstract

fetched live from OpenAlex

We study the mean molecular shape features for a model of wormlike chains with variable persistence length and nonbonded pair interactions. The chains are modelled as end-grafted and confined within an infinite slab with variable thickness. By using two independent shape properties (mean size and the complexity of chain entanglements), as well as a reference model with no attractive interactions (the self-avoiding walk), we propose an unbiased criterion to detect the formation of compact configurations. This process of compaction resembles qualitatively the onset of a “collapse transition” in a finite-size polymer. The method can be used even for short and medium-size chains, where scaling arguments are not applicable. We show that compaction occurs both for free mushrooms and strongly-confined chains. Moreover, the onset of compaction appears to depend little on the level of confinement. We find the same characteristic behaviour for either flexible or stiff chains, or for chains with interactions covering the range from good to poor solvent.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.014
Threshold uncertainty score0.987

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.022
GPT teacher head0.275
Teacher spread0.253 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations11
Published2001
Admission routes1
Has abstractyes

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