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Record W2040220553 · doi:10.1021/jp030434r

Luminescence Spectroscopy and Near-Infrared to Visible Upconversion of Nanocrystalline Gd<sub>3</sub>Ga<sub>5</sub>O<sub>12</sub>:Er<sup>3+</sup>

2003· article· en· W2040220553 on OpenAlexaff
Fiorenzo Vetrone, John‐Christopher Boyer, John A. Capobianco, Adolfo Speghini, Marco Bettinelli

Bibliographic record

VenueThe Journal of Physical Chemistry B · 2003
Typearticle
Languageen
FieldMaterials Science
TopicLuminescence Properties of Advanced Materials
Canadian institutionsConcordia University
Fundersnot available
KeywordsPhoton upconversionNanocrystalline materialInfraredExcitationLuminescenceSpectroscopyAnalytical Chemistry (journal)Materials scienceEnergy transferInfrared spectroscopyAtomic physicsOpticsChemistryOptoelectronicsPhysicsNanotechnology

Abstract

fetched live from OpenAlex

The near-infrared to visible upconversion properties of nanocrystalline Gd 3 Ga 5 O 12:Er 3+ (1 and 5%) were studied following excitation of the 4 I 9/2 exited state with 800 nm radiation. Intense green and red emissions were observed from the ( 2 H 11/2, 4 S 3/2 ) → 4 I 15/2 and 4 F 9/2 → 4 I 15/2 transitions, respectively. The upconverted decay times in the 1% sample were identical compared to those obtained with 488 nm excitation, indicating that ESA was responsible for populating the upper emitting states. However, as the Er 3+ concentration was increased to 5%, the upconverted decay times were lengthened and deviated from exponentiality, indicating the presence of energy transfer upconversion. In addition, an enhancement of the red ( 4 F 9/2 → 4 I 15/2 ) upconversion emission was observed in the 5% sample and occurred via an energy transfer process of the type ( 4 I 9/2, 4 I 11/2 ) → ( 4 I 13/2, 4 F 9/2 ).

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.001
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.001
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.000
Science and technology studies0.0000.001
Scholarly communication0.0000.001
Open science0.0010.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.007
GPT teacher head0.221
Teacher spread0.214 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations60
Published2003
Admission routes1
Has abstractyes

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