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Record W2041129638 · doi:10.1039/c4tc00451e

Evaluation of form birefringence in chiral nematic mesoporous materials

2014· article· en· W2041129638 on OpenAlexaff
Joel A. Kelly, C. P. K. Manchee, Susan Cheng, Jun Myun Ahn, Kevin E. Shopsowitz, Wadood Y. Hamad, Mark J. MacLachlan

Bibliographic record

VenueJournal of Materials Chemistry C · 2014
Typearticle
Languageen
FieldMaterials Science
TopicLiquid Crystal Research Advancements
Canadian institutionsFPInnovationsUniversity of TorontoUniversity of British Columbia
Fundersnot available
KeywordsBirefringenceMaterials scienceLiquid crystalRefractive indexCircular dichroismMesoporous materialCelluloseDichroismOpticsOptoelectronicsCrystallographyChemical engineeringOrganic chemistry

Abstract

fetched live from OpenAlex

We present a detailed investigation into the form birefringence of chiral nematic mesoporous materials templated by the self-assembly of cellulose nanocrystals as the potential basis to detect changes in refractive index in an optical sensor using circular dichroism (CD) spectroscopy. The behavior is in excellent agreement with a model of form birefringence in a chiral nematic structure. We characterize the variability introduced by the self-assembly of the biologically-derived cellulose nanocrystals, which can partially be accounted for through normalization to address reproducibility in thickness and helical pitch within each sample. As one potential application, we show that the refractive index performance of these materials is maintained in strongly absorbing solutions due to the chiral nature of the form birefringence.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.012
metaresearch head score (Gemma)0.002
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesInsufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.009
Threshold uncertainty score0.997

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0120.002
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0010.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0030.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.031
GPT teacher head0.326
Teacher spread0.295 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations21
Published2014
Admission routes1
Has abstractyes

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