MétaCan
Menu
Back to cohort
Record W2041153124 · doi:10.1103/physrevlett.91.048302

Photodestruction of Adenosine<mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"><mml:msup><mml:mn>5</mml:mn><mml:mo>′</mml:mo></mml:msup></mml:math>-Monophosphate (AMP) Nucleotide Ions<i>in vacuo</i>: Statistical versus Nonstatistical Processes

2003· article· lv· W2041153124 on OpenAlexaff
Steen Brøndsted Nielsen, J. U. Andersen, J.S. Forster, P. Hvelplund, B. Liu, U. V. Pedersen, S. Tomita

Bibliographic record

VenuePhysical Review Letters · 2003
Typearticle
Languagelv
FieldBiochemistry, Genetics and Molecular Biology
TopicAdvanced biosensing and bioanalysis techniques
Canadian institutionsUniversité de Montréal
Fundersnot available
KeywordsProtonationDeprotonationIonIntramolecular forceMaterials scienceChemistryStereochemistry

Abstract

fetched live from OpenAlex

The lifetimes of both deprotonated adenosine 5(')-monophosphate (AMP) and protonated AMP, after 266-nm photon absorption and intramolecular vibrational redistribution, were determined to be 16 micros based on a newly developed heavy-ion storage ring technique. Protonation of the adenine nucleobase seriously affects the fragmentation mechanism: the major part of the photoexcited anions fragment in a statistical (ergodic) process, whereas nearly all the cations (>99%) fragment in a nonergodic process. In solution at natural pH the AMP anion is prevalent and photoproduct formation is therefore less important as the time for vibrational cooling is of the order of picoseconds.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.002
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Theoretical or conceptual · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.916
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.002
Meta-epidemiology (narrow)0.0010.001
Meta-epidemiology (broad)0.0010.001
Bibliometrics0.0000.001
Science and technology studies0.0000.001
Scholarly communication0.0000.000
Open science0.0010.000
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.015
GPT teacher head0.275
Teacher spread0.261 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designTheoretical or conceptual
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations62
Published2003
Admission routes1
Has abstractyes

Explore more

Same venuePhysical Review LettersSame topicAdvanced biosensing and bioanalysis techniquesFrench-language works237,207