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Record W2043765535 · doi:10.1021/jp101176v

Differential Scanning Calorimetry Study of the Structure of Water Confined within AOT Lamellar Mesophases

2010· article· en· W2043765535 on OpenAlexaff
Éric Prouzet, Jean‐Blaise Brubach, Pascale Le Roy

Bibliographic record

VenueThe Journal of Physical Chemistry B · 2010
Typearticle
Languageen
FieldChemistry
TopicSurfactants and Colloidal Systems
Canadian institutionsUniversity of Waterloo
Fundersnot available
KeywordsDifferential scanning calorimetryLamellar structureBilayerPulmonary surfactantMaterials sciencePopulationCalorimetryCrystallographyChemical physicsAnalytical Chemistry (journal)ChemistryThermodynamicsChromatographyMembranePhysics

Abstract

fetched live from OpenAlex

We combined thermal analysis with FT-IR measurements to solve the structure of the water network confined within lamellar bilayers of AOT surfactant. Unlike previous FT-IR analyses that allowed us only to point out spectroscopic molecular components characterized by their local connectivity, differential scanning calorimetry (DSC) allowed us to identify homogeneous thermal populations listed as low, medium and high temperature. HT water was identified with bulk water, and LT water, as hydration water closely linked with surfactants heads. MT water was assigned to a disrupted network of water corresponding to a layer of 0.5 nm modified by the effect of confinement created by the vicinity of the surfactant bilayer. It appears from this study that the actual extent of confinement influence is lower than expected, at least for lamellar structures. Each thermal population was finally described by a different distribution of the spectroscopic components identified in parallel by FT-IR.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.002

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.007
GPT teacher head0.228
Teacher spread0.221 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations23
Published2010
Admission routes1
Has abstractyes

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Same venueThe Journal of Physical Chemistry BSame topicSurfactants and Colloidal SystemsFrench-language works237,207