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Record W2044238898 · doi:10.1002/chem.201490210

Cover Picture: Platinum Complexes of a Borane‐Appended Analogue of 1,1′‐Bis(diphenylphosphino)ferrocene: Flexible Borane Coordination Modes and in situ Vinylborane Formation (Chem. Eur. J. 51/2014)

2014· paratext· en· W2044238898 on OpenAlexaff
Bradley E. Cowie, David J. H. Emslie

Bibliographic record

VenueChemistry - A European Journal · 2014
Typeparatext
Languageen
FieldChemistry
TopicAsymmetric Hydrogenation and Catalysis
Canadian institutionsMcMaster University
Fundersnot available
KeywordsTrifluoromethylationElectrophileChemistryNucleophileBoraneReagentLigand (biochemistry)FerroceneCoordination complexPlatinumCombinatorial chemistryMedicinal chemistryStereochemistryCatalysisOrganic chemistryMetal

Abstract

fetched live from OpenAlex

An arylborane-appended analogue of the catalytically important dppf ligand, FcPPB, was prepared and is represented by the industrial robot in the image. FcPPB provided access to platinum complexes featuring η3BCC-, η2BC-, η1B- and Pt–H–B coordination modes, and reaction of the η3BCC-coordinated complex with PhC2H transformed the arylborane into an η3BCC-coordinated vinylborane. For details, see the Full Paper by B. E. Cowie and D. J. H. Emslie on pp. 16899 ff. (FcBBB=1′-{(ortho-diphenylborylphenyl)-tert-butylphosphino}-1-diphenylphosphinoferrocene)

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Not applicable · Consensus signal: none
GenreCandidate signal: Other · Consensus signal: Other
Teacher disagreement score0.125
Threshold uncertainty score0.417

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0010.000
Research integrity0.0010.001
Insufficient payload (model declined to judge)0.1250.013

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.012
GPT teacher head0.233
Teacher spread0.221 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designNot applicable
Domainnot available
GenreOther

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2014
Admission routes1
Has abstractyes

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Same venueChemistry - A European JournalSame topicAsymmetric Hydrogenation and CatalysisFrench-language works237,207