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Record W2047428186 · doi:10.1021/jp030413x

Alteration of Protein Constituents Induced by Low-Energy (<40 eV) Electrons. III. The Aliphatic Amino Acids

2003· article· en· W2047428186 on OpenAlexaff
Hassan Abdoul‐Carime, Léon Sanche

Bibliographic record

VenueThe Journal of Physical Chemistry B · 2003
Typearticle
Languageen
FieldChemistry
TopicMass Spectrometry Techniques and Applications
Canadian institutionsUniversité de Sherbrooke
Fundersnot available
KeywordsChemistryDissociation (chemistry)IonDesorptionPolyatomic ionCysteineElectronYield (engineering)CrystallographyAnalytical Chemistry (journal)Physical chemistryOrganic chemistryMaterials scienceAdsorptionEnzyme

Abstract

fetched live from OpenAlex

We report mass spectrometric measurements of anions desorbed by 1−40 eV electron impact on thin films of glycine (Gly), alanine (Ala) and cysteine (Cys) physisorbed on a Pt substrate. (H -, CH -, CH 2 -, CH 3 -, O -, OH -, and CN - ), (H -, CH 2 -, CH 3 -, O -, and OH - ), and (H -, O -, OH -, and CN -, S -, and SH - ) anions are observed to desorb from these irradiated molecular solids, respectively. The anion yield functions exhibit structures at energies below 15 eV, indicating that molecular dissociation operates via dissociative electron attachment (DEA). Above 15 eV, anion desorption is dominated principally by nonresonant dipolar dissociation (DD). However, an additional structure observed at 20 eV in the yield function of H - denotes the presence of a resonant process: DEA or decay of a transient molecular anion into the DD continuum or both. The presence of the sulfur group in cysteine enhances dissociation by 2 orders of magnitude relative to Gly and Ala.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.017
Threshold uncertainty score0.540

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.007
GPT teacher head0.239
Teacher spread0.232 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations34
Published2003
Admission routes1
Has abstractyes

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