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From structure topology to chemical composition. XI. Titanium silicates: crystal structures of innelite-1<i>T</i>and innelite-2<i>M</i>from the Inagli massif, Yakutia, Russia, and the crystal chemistry of innelite

2011· article· en· W2047763454 on OpenAlex

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affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.

Bibliographic record

VenueMineralogical Magazine · 2011
Typearticle
Languageen
FieldMaterials Science
TopicCrystal Structures and Properties
Canadian institutionsUniversity of Manitoba
Fundersnot available
KeywordsElectron microprobeMassifCrystal structureCrystallographyTitaniumGroup (periodic table)Crystal (programming language)Chemical compositionChemistryMaterials scienceMineralogyGeologyMetallurgyGeochemistry

Abstract

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Abstract The crystal structures of two polytypes of innelite, ideally Ba 4 Ti 2 Na 2 M 2+ Ti(Si 2 O 7 ) 2 [(SO 4 ) (PO 4 )]O 2 [O(OH)] where M 2+ = Mn, Fe 2+ , Mg, Ca: innelite-1T, a 5.4234(9), b 7.131(1), c 14.785(3) Å, α 98.442(4), β 94.579(3), γ 90.009(4)°, V 563.7(3) Å 3 , space group P1̄, D calc = 4.028 g/cm 3 , Z = 1; and innelite-2 M , a 5.4206(8), b 7.125(1), c 29.314(4) Å, 0 94.698(3)°, V 1128.3(2) Å 3 , space group P2/c, D calc. = 4.024 g/cm 3 , Z = 2, from the Inagli massif, Yakutia, Russia, have been refined to R values of 8.99 and 7.60%, respectively. Electron-microprobe analysis gave the empirical formula for innelite as (Ba 3.94 Sr 0.06 ) Σ4.00 (Na 2.16 Mn 0.38 2+ Fe 2+ 0.17 Mg 0.15 Ca 0.10 ☐ 0.04 ) Σ3 (Ti 2.97 Nb 0.02 Al 0.02 ) Σ3.01 Si 4.01 (S 1.02 P 0.81 ☐ 0.17 ) Σ2 H 1.84 O 25.79 F 0.21 which is equivalent to (Ba 3.94 Sr 0.06 ) Σ4.00 (Ti 1.97 Nb 0.02 Al0.02) Σ2.01 [(OH 0.99 F 0.21 ) Σ1.20 O 0.80 ], calculated on the basis of 26 (O + F) anions, with H 2 O calculated from structure refinement. The crystal structure of innelite is a combination of a TS (titanium silicate) block and an I (intermediate) block. The TS block consists of HOH sheets (H-heteropolyhedral, O-octahedral) and exhibits linkage and stereochemistry typical for Ti-disilicate minerals of Group III (Ti = 3 a.p.f.u.): two H sheets connect to the O sheet such that two (Si 2 O 7 ) groups link to the trans edges of a Ti octahedron of the O sheet. The I block contains T sites, statistically occupied by S and P, and Ba atoms. In the structures of innelite- 1T and innelite-2 M , TS blocks are related by an inversion centre and a c y glide plane, respectively. HRTEM images show a coherent intergrowth of the two polytypes, together with an as-yet unidentified ∼10 Å phase.

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Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesInsufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.269
Threshold uncertainty score0.999

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.000
Science and technology studies0.0000.002
Scholarly communication0.0000.000
Open science0.0010.001
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0020.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.014
GPT teacher head0.209
Teacher spread0.196 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it