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Record W2047853743 · doi:10.1021/je049949h

Determination of Vapor Pressures, Octanol−Air, and Water−Air Partition Coefficients for Polyfluorinated Sulfonamide, Sulfonamidoethanols, and Telomer Alcohols

2004· article· en· W2047853743 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.
fundA Canadian funder is recorded on the work.

Bibliographic record

VenueJournal of Chemical & Engineering Data · 2004
Typearticle
Languageen
FieldEnvironmental Science
TopicPer- and polyfluoroalkyl substances research
Canadian institutionsThe Scarborough HospitalUniversity of Toronto
FundersUniversity of Toronto
KeywordsChemistryPartition coefficientVolatility (finance)OctanolCarbon chainChromatographyVapor pressureOrganic chemistryAnalytical Chemistry (journal)

Abstract

fetched live from OpenAlex

Liquid-phase vapor pressures ( P L ) and octanol−air partition coefficients ( K OA ) for N- ethyl perfluorooctane sulfonamide, N- methyl perfluorooctanesulfonamidoethanol, N- ethyl perfluorooctanesulfonamidoethanol, and four fluorotelomer alcohols (CF 3 (CF 2 ) n CH 2 CH 2 OH, n = 3, 5, 7, and 9) were estimated as a function of temperature using a technique based on measuring gas chromatographic retention times relative to those of hexachlorobenzene. The method was calibrated using volatility data for fluorinated aromatic substances, chlorinated benzenes, and pesticides. The fluorinated telomer alcohols were found to have a volatility higher than that of the nonfluorinated alcohols of similar chain length and higher than that of perfluorinated aromatics of comparable molar mass. On the basis of their volatility, the polyfluorinated chemicals are expected to occur predominantly in the atmospheric gas phase. The water−air partition coefficient ( K WA ) for the three shorter carbon chain length fluorotelomer alcohols was determined as a function of temperature using equilibrium static headspace gas chromatography and the phase ratio variation method. The K WA values of the three fluorinated telomer alcohols extrapolated to 25 °C are of a similar order of magnitude (1 < log K WA < 2) and suggest that rain scavenging is not a very efficient atmospheric deposition process.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.013
Threshold uncertainty score0.427

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.021
GPT teacher head0.271
Teacher spread0.250 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it