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Record W2047931495 · doi:10.1115/gt2013-95151

Ignition Delay Time Experiments for Natural Gas/Hydrogen Blends at Elevated Pressures

2013· article· en· W2047931495 on OpenAlexaff
Marissa Brower, Olivier Mathieu, Eric L. Petersen, Nicola Donohoe, Alexander Heufer, Wayne K. Metcalfe, Henry J. Curran, Gilles Bourque, Felix Güthe

Bibliographic record

Venuenot available
Typearticle
Languageen
FieldChemical Engineering
TopicAdvanced Combustion Engine Technologies
Canadian institutionsRolls-Royce (Canada)
Fundersnot available
KeywordsHydrogenIgnition systemNatural gasHydrocarbonShock tubeEquivalence ratioChemistryAnalytical Chemistry (journal)Materials scienceThermodynamicsCombustionOrganic chemistryShock wavePhysics

Abstract

fetched live from OpenAlex

Applications of natural gases that contain high levels of hydrogen have become a primary interest in the gas turbine market. While the ignition delay times of hydrogen and of the individual hydrocarbons in natural gases can be considered well known, there have been few previous experimental studies into the effects of different levels of hydrogen on the ignition delay times of natural gases at gas turbine conditions. To examine the effects of hydrogen content at gas turbine conditions, shock-tube experiments were performed on nine mixtures of an L9 matrix. The L9 matrix was developed by varying four factors: natural gas higher-order hydrocarbon content of 0, 18.75, or 37.5%; hydrogen content of the total fuel mixture of 30, 60, or 80%; equivalence ratios of 0.3, 0.5, or 1; and pressures of 1, 10, or 30 atm. Temperatures ranged from 1092 K to 1722 K, and all mixtures were diluted in 90% Ar. Correlations for each mixture were developed from the ignition delay times and, using these correlations, a factor sensitivity analysis was performed. It was found that hydrogen played the most significant role in the ignition delay times of a mixture. Pressure was almost as important as hydrogen content, especially as temperature increased. Equivalence ratio was slightly more important than hydrocarbon content of the natural gas, but both were less important than pressure or hydrogen content. Comparison with a modern chemical kinetic model demonstrated that the model captures well the relative impacts of H2 content, temperature, and pressure, but some improvements are still needed in terms of absolute ignition delay times.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesInsufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.230
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.011
GPT teacher head0.241
Teacher spread0.231 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations8
Published2013
Admission routes1
Has abstractyes

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