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Improved Density Prediction for Mixtures of Native and Refined Heavy Oil with Solvents

2015· article· en· W2051708725 on OpenAlexafffund
M. C. Sánchez-Lemus, J. C. Okafor, D. P. Ortiz, F. F. Schoeggl, Shawn D. Taylor, Frans G. A. van den Berg, Harvey W. Yarranton

Bibliographic record

VenueEnergy & Fuels · 2015
Typearticle
Languageen
FieldEngineering
TopicPhase Equilibria and Thermodynamics
Canadian institutionsSchlumberger (Canada)University of Calgary
FundersNatural Sciences and Engineering Research Council of CanadaVirtual Materials GroupPetrobrasChina National Offshore Oil CorporationShell
KeywordsTolueneChemistryAsphalteneNaphthaHydrocarbonDistillationFraction (chemistry)HeptaneHydrocarbon mixturesMixing (physics)Diesel fuelBenzeneVolume (thermodynamics)Analytical Chemistry (journal)Mass fractionThermodynamicsChromatographyOrganic chemistry

Abstract

fetched live from OpenAlex

A correlation was developed to predict the density of mixtures of heavy oil (and other petroleum liquids) and hydrocarbon solvents when the densities of each fluid in the mixture are available. Densities at atmospheric pressure and 293 K were measured for saturates and aromatics (SA) fractions from 10 native, thermo-cracked, and hydrocracked heavy oils all mixed with toluene and n -heptane; distillation cuts from 6 heavy oils mixed with toluene; and mixtures of deasphalted heavy oils with naphtha, diesel, and condensate. Density of mixtures of hydrocarbons and solvents at higher pressures (0.1–10 MPa) and temperatures (298–353 K) were also measured or obtained from the literature. Symmetry versus mass fraction was observed for all of the mixtures, and their densities were fitted with a mixing rule in which excess volumes are quantified with a binary interaction parameter and the density of each mixture component. The excess volume mixing rule fit the data for each mixture with average absolute deviations (AAD) less than 1.1 kg/m 3, and the overall average AAD was 0.39 kg/m 3 . The binary interaction parameter was correlated to the density of the components in the mixture and to temperature. Pressure was found to have no consistent effect in the interaction parameter and was neglected. The overall AAD for the density determined with the correlated β 12 for binary mixtures was 1.1 kg/m 3 compared with 3.0 kg/m 3 if regular solution behavior was assumed and 3.6 kg/m 3 when the standard American Petroleum Institute (API) correlation was used to predict the density of the mixtures. The API correlation and correlated excess volume mixing rule performed similarly for hydrocarbons with carbon numbers above five. The proposed correlation was also tested on ternary data from the literature with comparable results.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.134
Threshold uncertainty score0.306

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.010
GPT teacher head0.207
Teacher spread0.197 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations12
Published2015
Admission routes2
Has abstractyes

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