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Record W2051818035 · doi:10.1021/ef700424k

Production of Heavy Oils with High Caloric Values by Direct Liquefaction of Woody Biomass in Sub/Near-critical Water

2007· article· en· W2051818035 on OpenAlexaff
Chunbao Xu, Nimisha Lad

Bibliographic record

VenueEnergy & Fuels · 2007
Typearticle
Languageen
FieldEngineering
TopicSubcritical and Supercritical Water Processes
Canadian institutionsLakehead University
Fundersnot available
KeywordsLiquefactionChemistryCatalysisSawdustYield (engineering)Biomass (ecology)Heat of combustionPulp and paper industryNuclear chemistryOrganic chemistryAgronomyMaterials scienceMetallurgy

Abstract

fetched live from OpenAlex

Direct liquefaction of a woody biomass (Jack pine sawdust) in sub/near-critical water without and with catalysts (alkaline earth and iron ions) has been investigated at temperatures of 280–380 °C. Heavy oils with a high caloric value of 30–35 MJ/kg (much greater than that of the crude wood sample used) were obtained, along with water soluble oils with a caloric value of 19–25 MJ/kg. The yields of heavy oil and total oil products tended to maximize in the temperature range of 280–340 °C for all the liquefaction operations regardless of the presence of a catalyst or the type of catalyst. All the catalysts tested, i.e., Ca(OH) 2, Ba(OH) 2, and FeSO 4, were found effective for enhancing the formation of heavy oil products at 280–340 °C, while they significantly promoted the formation of gas and water at >340 °C. The yield of heavy oil in the operation at 300 °C for 30 min was improved significantly from around 30% without catalyst to greater than 45% by Ba(OH) 2 . The maximum yield of total oil products reached 51% in the operation without catalyst, while it increased to about 65% with Ca(OH) 2 at 300 °C. The GC/MS measurements for the heavy oil products revealed that the oils contain mainly carboxylic acids, phenolic compounds and derivatives, and long-chain alkanes.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.002

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.006
GPT teacher head0.208
Teacher spread0.202 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations213
Published2007
Admission routes1
Has abstractyes

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