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Record W2053197962 · doi:10.1039/c5nr00561b

Photoluminescent silicon nanocrystal-polymer hybrid materials via surface initiated reversible addition–fragmentation chain transfer (RAFT) polymerization

2015· article· en· W2053197962 on OpenAlexaff
Ignaz M. D. Höhlein, Patrick D. L. Werz, Jonathan G. C. Veinot, Bernhard Rieger

Bibliographic record

VenueNanoscale · 2015
Typearticle
Languageen
FieldMaterials Science
TopicSilicon Nanostructures and Photoluminescence
Canadian institutionsUniversity of Alberta
Fundersnot available
KeywordsChain transferRaftPhotoluminescencePolymerMaterials sciencePolymerizationReversible addition−fragmentation chain-transfer polymerizationMonomerChemical engineeringPolymer chemistrySiliconNanocrystalPhotochemistryNanotechnologyRadical polymerizationChemistryOptoelectronicsComposite material

Abstract

fetched live from OpenAlex

Silicon-polymer core-shell hybrid materials are obtained via surface initiated reversible addition-fragmentation chain transfer (RAFT) polymerization from photoluminescent silicon nanocrystals (SiNCs). Polymer grafted SiNCs and free polymers in solution are separated using ultracentrifugation. The polymerization on the surface proceeds in a living manner which is confirmed via GPC, DLS and TGA measurements. This method was applied to various other monomers. The obtained materials all show bright red photoluminescence originating from the SiNC core.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow), Insufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.004
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.001
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0040.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.021
GPT teacher head0.242
Teacher spread0.221 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations20
Published2015
Admission routes1
Has abstractyes

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