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Record W2055027950 · doi:10.1002/cjce.20498

Kinetics study on cnt‐supported RuKCo FTS catalyst in a fixed bed reactor

2011· article· en· W2055027950 on OpenAlexafffundvenue
Mariane Trépanier, Christopher A. Dorval Dion, Ajay K. Dalai, Nicolas Abatzoglou

Bibliographic record

VenueThe Canadian Journal of Chemical Engineering · 2011
Typearticle
Languageen
FieldChemical Engineering
TopicCatalysts for Methane Reforming
Canadian institutionsUniversité de SherbrookeUniversity of Saskatchewan
FundersEnerkem
KeywordsMicroreactorCatalysisSpace velocityFischer–Tropsch processThermodynamicsKineticsActivation energySyngasChemistryRate equationKinetic energyReaction rateChemical kineticsPhysical chemistryMaterials sciencePhysicsOrganic chemistryClassical mechanics

Abstract

fetched live from OpenAlex

Abstract The rate of syngas (H 2 /CO) consumption over a RuKCo/CNT Fischer–Tropsch synthesis (FTS) catalyst was measured in a fixed bed microreactor at 210–225°C, 2–3.5 MPa, H 2 /CO feed molar ratios of 1–2.5, and gas hourly space velocity (GHSV) range of 2700–3600 h −1 . The data have been used to model the kinetics of the FTS reactions within the range of the studied conditions. One empirical power law model and four semi‐empirical kinetic models based on Langmuir–Hinshelwood‐type equation have been evaluated. The best fitting was obtained with the equation: similar to that proposed by Brötz et al. The estimated activation energy ( E = 80–85 kJ/mol) is lower than that is reported in the literature. The validity of these results are restricted to fixed beds with the given catalyst in the tested conversion regime.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.001
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.004
Threshold uncertainty score0.903

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.001
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.001
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0010.000
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.024
GPT teacher head0.216
Teacher spread0.193 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations4
Published2011
Admission routes3
Has abstractyes

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