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Record W2055904118 · doi:10.1016/j.fuel.2014.11.008

Thermodynamic effects of calcium and iron oxides on crystal phase formation in synthetic gasifier slags containing from 0 to 27 wt.% V2O3

2014· article· en· W2055904118 on OpenAlexafffund
Jinichiro Nakano, Marc Duchesne, James Bennett, Kyei‐Sing Kwong, Anna Nakano, Robin W. Hughes

Bibliographic record

VenueFuel · 2014
Typearticle
Languageen
FieldEngineering
TopicMetallurgical Processes and Thermodynamics
Canadian institutionsNatural Resources Canada
FundersOffice of Energy Research and DevelopmentNational Energy Technology LaboratoryNatural Sciences and Engineering Research Council of CanadaOak Ridge Institute for Science and EducationNatural Resources CanadaU.S. Department of Energy
KeywordsVanadiumIsothermal processSlag (welding)MeliliteElectron microprobeMaterials scienceAnalytical Chemistry (journal)MullitePhase (matter)Phase diagramFayaliteCokeCalcium oxideMetallurgyChemistryMineralogyOlivineThermodynamicsSpinelCeramic

Abstract

fetched live from OpenAlex

Thermodynamic phase equilibria in synthetic slags (Al 2 O 3 –CaO–FeO–SiO 2 –V 2 O 3 ) were investigated with 0–27 wt.% vanadium oxide corresponding to industrial coal–petroleum coke (petcoke) feedstock blends in a simulated gasifier environment. Samples encompassing coal–petcoke mixed slag compositions were equilibrated at 1500 °C in a 64 vol.% CO/36 vol.% CO 2 atmosphere ( P o 2 ≈ 10 −8 atm at 1500 °C) for 72 h, followed by rapid water quench, then analyzed by inductively coupled plasma optical emission spectrometry, X-ray diffractometry, and scanning electron microscopy with wavelength dispersive spectroscopy. With increasing CaO content, FeO content, or both; the slag homogeneity region expanded and a composition range exhibiting crystals was reduced. The mullite (Al 6 Si 2 O 13 ) crystalline phase was not present in the slags above 9 wt.% FeO while the karelianite (V 2 O 3 ) crystalline phase was always present in compositions studied if a sufficient amount of vanadium existed in the slag. Based on the present experimental equilibrium evaluation, a set of isothermal phase diagrams showing effects of CaO and FeO on thermodynamic phase stabilities in the vanadium-bearing slags is proposed. Some uses of the diagrams for potential industrial practice are discussed.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Simulation or modeling · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.951
Threshold uncertainty score0.462

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.007
GPT teacher head0.222
Teacher spread0.215 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designSimulation or modeling
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations38
Published2014
Admission routes2
Has abstractyes

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