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Record W2057465882 · doi:10.2118/168070-ms

Frequency Dependent Magnetic Resonance Response of Heavy Crude Oils: Methods and Applications

2013· article· en· W2057465882 on OpenAlexaff
Arjun Kurup, Andrea Valori, H. N. Bachman, Jean‐Pierre Korb, Martin D. Hürlimann, Łukasz Zieliński

Bibliographic record

Venuenot available
Typearticle
Languageen
FieldPhysics and Astronomy
TopicNMR spectroscopy and applications
Canadian institutionsSchlumberger (Canada)
Fundersnot available
KeywordsAsphalteneDispersion (optics)Relaxation (psychology)Crude oilNuclear magnetic resonanceMaterials scienceRange (aeronautics)Analytical Chemistry (journal)ChemistryPetroleum engineeringGeologyChromatographyOrganic chemistryComposite materialPhysics

Abstract

fetched live from OpenAlex

Abstract Oilfield nuclear magnetic resonance (NMR) applications are widely accepted for characterizing reservoir rocks and fluids. All of the downhole applications, and most oilfield NMR lab work, are carried out assuming that the results are independent of the operating frequency. The assumption is generally warranted, since most NMR logging tools and lab devices operate in the 0.5 to 2 MHz range. However, two strong motivations exist for investigating the frequency dependence (that is, dispersion) of NMR of crude oil samples: 1) introduction and acceptance of lower frequency logging while drilling (LWD) and multi- frequency wireline NMR tools, and 2) sensitivity of NMR dispersion to the interaction and dynamics of molecules of varying size in complex fluids. We report here on a versatile frequency-dependent lab NMR measurement known as fast field cycling (FFC) NMR. The results clearly demonstrate a frequency dependence of the longitudinal relaxation time, T1, for crude oils between 10 kHz and 40 MHz. The study investigates the full T1 distributions for crude oils containing significant amounts of all the SARA (saturates, aromatics, resins, asphaltene) fractions, including a broad range of concentrations for the heavier fractions. For crude oils containing minimal asphaltene and resin fractions, the dispersion is minimal. In contrast, crude oils containing larger concentrations of asphaltene and resins show a clear shift of the T1 distribution to longer times at higher frequencies. We will discuss the implications and benefits of NMR dispersion for oilfield application. We suggest how the dispersion can be understood in terms of the molecular dynamics of asphaltenes with the rest the oil. Finally, we will provide an overview of the experimental challenges in making these measurements, including the hardware design and the specialized pulse sequences required for acquiring multi-frequency data.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesInsufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.310
Threshold uncertainty score0.999

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0020.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.010
GPT teacher head0.353
Teacher spread0.343 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations6
Published2013
Admission routes1
Has abstractyes

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