Autler-Townes Effects in Attosecond Circular Polarization Molecular Photoionization
Bibliographic record
Abstract
We present molecular photoionization simulations by intense (I ~ 1016 W/cm2) few cycle circularly polarized attosecond extreme ultraviolet laser pulses for aligned H2+ from numerical solutions of the corresponding time-dependent Schrodinger equation. With appropriate laser pulse parameters, circular attosecond coherent electron wave packets (CEWPs) are created in excited Rydberg states. Such CEWPs are spatially localized during ionization processes, thus resulting in sufficient population oscillations between the resonant excited Rydberg states and the initial ground state. Consequently Autler-Townes splitting in circular polarization energy spectra is predicted, which is shown to be critically sensitive to the pulse intensity, duration, and polarization. The resulting photoelectron angular distributions are rotated with respect to the molecular axis due to the nonspherical Coulomb potential of the molecule, resulting in different ionization rates at different laser polarization-molecular angles.
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How this classification was reachedexpand
Full frame distilled prediction
Teacher imitationNot calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.
Codex and Gemma teacher scores by category
| Category | Codex | Gemma |
|---|---|---|
| Metaresearch | 0.000 | 0.000 |
| Meta-epidemiology (narrow) | 0.000 | 0.000 |
| Meta-epidemiology (broad) | 0.000 | 0.000 |
| Bibliometrics | 0.000 | 0.000 |
| Science and technology studies | 0.000 | 0.000 |
| Scholarly communication | 0.000 | 0.001 |
| Open science | 0.000 | 0.000 |
| Research integrity | 0.000 | 0.000 |
| Insufficient payload (model declined to judge) | 0.000 | 0.000 |
Machine scores (provisional)
The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.
Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.
score_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from itClassification
machine, unvalidatedMachine predicted; a candidate call from one teacher head, not a consensus.
How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".