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Record W2060236946 · doi:10.1086/430084

Laboratory and Theoretical Simulation of 3.4 μm Spectra of Hydrocarbons in Interstellar Sources

2005· article· en· W2060236946 on OpenAlexaff
W. W. Duley, Victor I. Grishko, J. Kenel, G. R. Lee-Dadswell, Andrew D. Scott

Bibliographic record

VenueThe Astrophysical Journal · 2005
Typearticle
Languageen
FieldChemistry
TopicSpectroscopy and Laser Applications
Canadian institutionsUniversity of GuelphUniversity of Waterloo
Fundersnot available
KeywordsPhysicsSpectral lineAstrophysicsAstrochemistryInterstellar mediumMolecular cloudAmorphous carbonInterstellar cloudCarbon fibersAmorphous solidCosmic dustMoleculeHydrocarbonAbsorption (acoustics)Spectral bandsInfraredInfrared spectroscopyAstronomyGalaxyStarsCrystallographyComposite numberChemistryMaterials scienceOpticsOrganic chemistry

Abstract

fetched live from OpenAlex

The presence of hydrocarbons in interstellar clouds and in some emission objects can be inferred from the appearance of spectral features near 3.4 μm that are characteristic of CH2 and CH3 groups. While the 3.4 μm band attributable to these hydrocarbons has been found to be similar in sources such as GC IRS 6E and CRL 618 (Chiar et al. 1998), there are significant variations in the relative amplitude of individual components in other sources such as NGC 7538 IRS9 (Allamandola et al. 1992). This indicates that the composition of these hydrocarbons may depend on ambient conditions in interstellar clouds. To investigate this possibility, we have analyzed observational IR spectra of GC IRS 6E, CRL 618, IRAS 05341+0852, and NGC 7538 IRS9 to extract spectral bands associated with CH2 and CH3 groups in each of these sources. These components are compared with the features that appear in laboratory absorption and emission spectra of hydrogenated amorphous carbon. It is found that significant differences exist in the CH2/CH3 ratio in individual sources. In particular, we find that CH3 groups are suppressed in dense cloud dust but that CH2 groups are still abundant. The properties of individual spectral components within the 3.4 μm interstellar band are discussed and compared to laboratory and theoretical data on IR spectra of certain hydrocarbon molecules, as well as that of hydrogenated amorphous carbon. Simulation of 3.4 μm spectra using a random covalent network model is shown to provide a useful way to extract structural and bonding information for specific chemical groups in interstellar material.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.098
Threshold uncertainty score0.201

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.004
GPT teacher head0.237
Teacher spread0.233 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations18
Published2005
Admission routes1
Has abstractyes

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