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Record W2060820618 · doi:10.1002/3527606548.ch6

Recent Advances in the Preparation of Allylboronates and Their Use in Tandem Reactions with Carbonyl Compounds

2005· other· en· W2060820618 on OpenAlexaff
Jason W. J. Kennedy, Dennis G. Hall

Bibliographic record

Venuenot available
Typeother
Languageen
FieldChemistry
TopicOrganoboron and organosilicon chemistry
Canadian institutionsUniversity of Alberta
Fundersnot available
KeywordsChemistryAllylic rearrangementTandemIntramolecular forceMetathesisOrganic chemistryCatalysisPolymerization

Abstract

fetched live from OpenAlex

This chapter contains sections titled: Introduction Preparation of Allylboronates Direct Methods Allylboronates from Allylmetal Intermediates Allylboronates from Alkenylmetal Intermediates Allylboronates from the Hydroboration of 1,3-Butadienes and Allenes Allylboronates from the Transition-metal Catalyzed Diboration and Silaboration of Dienes and Allenes Allylboronates from Palladium-catalyzed Cross-coupling Reactions with Alkenyl Fragments Allylboronates from Palladium-catalyzed Cross-coupling Reactions with Allyl Electrophiles Indirect Methods Allylboronates from Alcoholysis of Triallylboranes Allylboronates from Homologation of Alkenylboronates Allylboronates from Allylic Rearrangement of Alkenylboronates Allylboronates from Isomerization of Alkenylboronates Allylboronates by Cycloadditions of Dienylboronates Allylboronates by Olefin Metathesis Reactions of Allylboronates Additions to Aldehydes – Formation of Homoallylic Alcohols Stereoselectivity and Mechanism of Non-catalyzed Additions Lewis Acid-catalyzed Additions Stereoselective Additions with Chiral Allylboronates Additions to Ketones Additions to Imine Derivatives Applications of Allylboronates in Tandem Reactions with Carbonyl Compounds Allylboration as the Terminal Process Tandem [4+2] Cycloaddition/Allylation Tandem Hydroformylation/Intramolecular Allylation Tandem Alkene Cross-metathesis/Allylation Tandem Diene Hydroboration/Allylation Tandem Diene Diborylation (Silaboration)/Allylboration Tandem Allylic Borylation/Intramolecular Allylation Allylboration as the Initiating Process Tandem Allylation/Allylation Tandem Allylation/Lactonization Tandem Allylation/Dioxene Thermolysis Conclusion References

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Not applicable · Consensus signal: none
GenreCandidate signal: Other · Consensus signal: none
Teacher disagreement score0.005
Threshold uncertainty score0.017

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0010.001
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0010.001
Science and technology studies0.0000.000
Scholarly communication0.0010.001
Open science0.0010.001
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0050.003

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.010
GPT teacher head0.250
Teacher spread0.240 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designNot applicable
Domainnot available
GenreOther

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations25
Published2005
Admission routes1
Has abstractyes

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