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Record W2060978473 · doi:10.1002/chem.201490090

Back Cover: Ruthenium Complexes of an Abnormally Bound, Anionic N‐Heterocyclic Carbene (Chem. Eur. J. 22/2014)

2014· paratext· en· W2060978473 on OpenAlexaff
Conor Pranckevicius, Douglas W. Stephan

Bibliographic record

VenueChemistry - A European Journal · 2014
Typeparatext
Languageen
FieldChemistry
TopicCatalytic Cross-Coupling Reactions
Canadian institutionsUniversity of Toronto
Fundersnot available
KeywordsRutheniumCarbeneChemistryLigand (biochemistry)Medicinal chemistryPolymer chemistryStereochemistryOrganic chemistryCatalysisReceptor

Abstract

fetched live from OpenAlex

The silver complex of an abnormally bound, anionic N-heterocyclic carbene (NHC) can be transmetalated to ruthenium. The resulting ruthenium complexes are rare examples of anionic NHCs on ruthenium. Although Ru binding to the abnormal position of the carbene is observed in the complexes Ru(IDipp-BF3)(p-cymene)(L)Cl (IDipp-BF3=1,3-(2,6-iPr2C6H3)2-2-BF3(C3HN2)-4-yl), abstraction of chloride results in the unprecedented binding of the carbene via the methine position of the IDipp-BF3 ligand. For more information, see the Communication by D. W. Stephan and C. Pranckevicius on page 6597 ff.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow), Research integrity, Insufficient payload (model declined to judge)
Consensus categoriesInsufficient payload (model declined to judge)
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.314
Threshold uncertainty score0.999

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0010.001
Meta-epidemiology (broad)0.0010.001
Bibliometrics0.0000.000
Science and technology studies0.0010.001
Scholarly communication0.0010.000
Open science0.0020.001
Research integrity0.0010.004
Insufficient payload (model declined to judge)0.0580.011

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.014
GPT teacher head0.255
Teacher spread0.241 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; both teacher heads agree on what is shown here.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2014
Admission routes1
Has abstractyes

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