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Record W2061591889 · doi:10.1063/1.1603732

Enantiomeric purification of nonpolarized racemic mixtures using coherent light

2003· article· en· W2061591889 on OpenAlexaff
Einat Frishman, Moshe Shapiro, David Gerbasi, Paul Brumer

Bibliographic record

VenueThe Journal of Chemical Physics · 2003
Typearticle
Languageen
FieldPhysics and Astronomy
TopicLaser-Matter Interactions and Applications
Canadian institutionsUniversity of TorontoUniversity of British Columbia
Fundersnot available
KeywordsEnantiomerPolarization (electrochemistry)Angular momentumDipolePhysicsLaserRacemic mixtureProjection (relational algebra)Total angular momentum quantum numberOpticsChemistryQuantum mechanicsStereochemistryPhysical chemistryMathematicsAlgorithm

Abstract

fetched live from OpenAlex

Angular momentum constraints for coherently controlling chiral purification of racemic mixtures using the dipole-electric field interaction are examined in detail for two different scenarios. First shown is that achieving enantiomeric control in our earlier scheme [M. Shapiro, E. Frishman, and P. Brumer, Phys. Rev. Lett. 84, 1669 (2000)], using parallel laser pulses, requires that the system be M-polarized, where M is the projection of the total angular momentum along the axis of laser polarization. An alternate scenario is then introduced that allows chiral control in an unpolarized racemic mixture by using three mutually perpendicular linearly polarized light fields. Analytic expressions for the enantiomeric excess in both cases are derived and computational results are presented.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.046
Threshold uncertainty score0.224

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.015
GPT teacher head0.271
Teacher spread0.256 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations31
Published2003
Admission routes1
Has abstractyes

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