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Record W2063190707 · doi:10.1039/b008013f

The determination of six taste and odour compounds in water using Ambersorb 572 and high resolution mass spectrometry

2001· article· en· W2063190707 on OpenAlexaff
J-P.F.P. Palmentier, Vince Y. Taguchi

Bibliographic record

VenueThe Analyst · 2001
Typearticle
Languageen
FieldChemistry
TopicAnalytical chemistry methods development
Canadian institutionsMinistry of the Environment, Conservation and Parks
Fundersnot available
KeywordsGeosminChemistryChromatographyMass spectrometryOrbitrapDetection limitGas chromatography–mass spectrometryGas chromatographyOdorOrganic chemistry

Abstract

fetched live from OpenAlex

A method for the analysis of six taste and odour causing compounds in aqueous samples using the granular adsorbent, Ambersorb 572, and gas chromatography-high resolution mass spectrometry (GC-HRMS) has been developed. This method for the determination of geosmin, 2-methylisoborneol (2-MIB), 2-isopropyl-3-methoxypyrazine (IPMP), 2-isobutyl-3-methoxypyrazine (IBMP), 2,3,6-trichloroanisole (236-TCA) and 2,4,6-trichloroanisole (246-TCA) is highly productive [up to 40 samples per day + 23 quality control (QC) samples] and provides rapid (24-48 h) turnaround times. The analytes are extracted from water by the addition of Ambersorb 572 to the sample bottle and rolling for 1 h. The adsorbent is isolated by filtration and allowed to air dry for 1 h. The Ambersorb 572 is transferred to an autosampler vial and the analytes are desorbed into dichloromethane. The extract is analysed by GC-HRMS at 7000 resolving power (RP). Quantification is performed by isotope dilution and internal standard techniques utilizing d3-geosmin, d3-2-MIB, d5-246-TCA and 2-sec-butyl-3-methoxypyrazine (s-BMP). Method precisions of 3.5-5.8% and accuracies of +/- 5.7-8.9% were obtained. Reporting detection limits (RDLs) of 1.0 ng L-1 were obtained for 2-MIB, geosmin, IPMP and IBMP, while RDLs of 2.0 ng L-1 were obtained for 236-TCA and 246-TCA.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.088
Threshold uncertainty score0.249

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.033
GPT teacher head0.282
Teacher spread0.249 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations21
Published2001
Admission routes1
Has abstractyes

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