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Record W2064289896 · doi:10.1515/pac-2013-1023

Assessment of international reference materials for isotope-ratio analysis (IUPAC Technical Report)

2014· article· en· W2064289896 on OpenAlexfundno aff
Willi A. Brand, Tyler B. Coplen, Jochen Vogl, Martin Rösner, Thomas Prohaska

Bibliographic record

VenuePure and Applied Chemistry · 2014
Typearticle
Languageen
FieldChemistry
TopicRadioactive element chemistry and processing
Canadian institutionsnot available
FundersArgonne National LaboratoryNational Research Council CanadaNational Institute of Standards and TechnologyU.S. Geological SurveyInternational Atomic Energy AgencyUniversity of CalgaryU.S. Department of Energy
KeywordsChemical nomenclatureNatural abundanceDeltaIsotopeChemistryIsotope analysisStable isotope ratioIsotope geochemistryInstrumentation (computer programming)Environmental chemistryMineralogyEarth scienceAnalytical Chemistry (journal)RadiochemistryGeologyNuclear physicsPhysics

Abstract

fetched live from OpenAlex

Abstract Since the early 1950s, the number of international measurement standards for anchoring stable isotope delta scales has mushroomed from 3 to more than 30, expanding to more than 25 chemical elements. With the development of new instrumentation, along with new and improved measurement procedures for studying naturally occurring isotopic abundance variations in natural and technical samples, the number of internationally distributed, secondary isotopic reference materials with a specified delta value has blossomed in the last six decades to more than 150 materials. More than half of these isotopic reference materials were produced for isotope-delta measurements of seven elements: H, Li, B, C, N, O, and S. The number of isotopic reference materials for other, heavier elements has grown considerably over the last decade. Nevertheless, even primary international measurement standards for isotope-delta measurements are still needed for some elements, including Mg, Fe, Te, Sb, Mo, and Ge. It is recommended that authors publish the delta values of internationally distributed, secondary isotopic reference materials that were used for anchoring their measurement results to the respective primary stable isotope scale.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.076
metaresearch head score (Gemma)0.052
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Not applicable · Consensus signal: none
GenreCandidate signal: Other · Consensus signal: none
Teacher disagreement score0.076
Threshold uncertainty score0.400

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0760.052
Meta-epidemiology (narrow)0.0040.001
Meta-epidemiology (broad)0.0020.002
Bibliometrics0.0240.016
Science and technology studies0.0030.002
Scholarly communication0.0070.004
Open science0.0100.005
Research integrity0.0050.004
Insufficient payload (model declined to judge)0.0140.024

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.013
GPT teacher head0.303
Teacher spread0.291 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designNot applicable
Domainnot available
GenreOther

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations687
Published2014
Admission routes1
Has abstractyes

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