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Record W2064317306 · doi:10.2118/81203-ms

A Novel Approach to Hydrogen Sulfide Removal From Natural Gas

2003· article· en· W2064317306 on OpenAlexaff
Brandy Fidler, Kerry L. Sublette, G. E. Jenneman, Greg A. Bala

Bibliographic record

VenueSPE/EPA/DOE Exploration and Production Environmental Conference · 2003
Typearticle
Languageen
FieldChemical Engineering
TopicOdor and Emission Control Technologies
Canadian institutionsConocoPhillips (Canada)
Fundersnot available
KeywordsHydrogen sulfideSulfideThiosulfateSulfate-reducing bacteriaSulfurChemistryEnvironmental chemistryWaste managementNatural gasBiomass (ecology)BioreactorSour gasPulp and paper industrySulfateOrganic chemistryGeology

Abstract

fetched live from OpenAlex

Abstract Sulfide removal is a significant problem in the oil and gas industry. Some of the problems presented by sulfides include environmental compliance, toxicity, corrosion, reduced efficiency of fluid handling equipment, offensive odor, reduced value of products, and increased operation costs. Microbial oxidation of sulfides offers the potential for a safe, cost-effective method of removing sulfides from natural gas, sour water, spent-sulfidic caustic, etc. The purpose of this study is the development of an efficient and economically viable bioreactor system for sulfide oxidation. The application of immediate interest is the removal of H2S from "stranded" natural gas. The immobilization matrix Bio-Sep® has previously been used for successful biotreatment of BTEX-contaminated groundwater. In this study, a special sorbent has been added to Bio-Sep® to adsorb sulfide while still maintaining the desirable physical properties of the original beads. Thiobacillus denitrificans is a sulfide-oxidizing autotroph which may use either oxygen or nitrate as a terminal electron acceptor. Thiosulfate, elemental sulfur, or sulfide may be used as an energy source for T. denitrificans and each are oxidized to sulfate. Previously, suspended cultures of T. denitrificans were shown to remove H2S from a gas stream with 1-2 s of gas-liquid contact time. However, the volumetric productivity of suspended cultures was insufficient to lead to an economically viable bioreactor design due to low biomass concentrations. In order to increase biomass concentration and volumetric productivity T. denitrificans has been immobilized in both standard Bio-Sep® and the new sulfide-sorbing version (Bio-Sep®S). The two matrices will be compared according to their ability to immobilize this sulfide-oxidizing culture and increase biomass concentration and volumetric productivity.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.102
Threshold uncertainty score0.889

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.031
GPT teacher head0.215
Teacher spread0.184 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations6
Published2003
Admission routes1
Has abstractyes

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