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A TiO<sub>2</sub>nanostructure transformation: from ordered nanotubes to nanoparticles

2009· article· en· W2065246045 on OpenAlexfundno aff
Yahya Alivov, Zhaoyang Fan

Bibliographic record

VenueNanotechnology · 2009
Typearticle
Languageen
FieldEnergy
TopicTiO2 Photocatalysis and Solar Cells
Canadian institutionsnot available
FundersUniversity of California, IrvineRyerson University
KeywordsMaterials scienceAmorphous solidNanoparticleChemical engineeringEthylene glycolAnnealing (glass)NanotubeNanostructureNanotechnologyElectrolytePhotoluminescenceTetragonal crystal systemTitanium dioxideCrystal structureCrystallographyComposite materialOptoelectronicsPhysical chemistryCarbon nanotube

Abstract

fetched live from OpenAlex

Transformation of TiO2 nanotubes (NTs) to truncated tetragonal bipyramidal shape nanoparticles (NPs) was observed upon thermally annealing titanium dioxide (TiO2) ordered nanotube arrays in fluorine ambient, resulting from the reaction of fluorine ions (F(-)) from the electrolyte residues in long nanotubes grown by anodization in ethylene glycol+NH4F electrolyte. The size of the TiO2 nanoparticles formed depends on the fluorine concentration and can be controlled from 20 to 500 nm. The crystal and optical properties of the nanoparticle layers are superior compared with those of nanotube arrays which are also annealed but without undergoing a morphology transformation, as was shown by means of x-ray diffraction and photoluminescence spectroscopy measurements. The NT-NP transformation mechanism was studied by analyzing the initial stages of the NT-NP transformation. This was achieved by terminating the annealing process in F ambient after 1-5 min. It was found that amorphous NTs first contract, then break down, and finally merge and crystallize to form NPs.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.003

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.007
GPT teacher head0.210
Teacher spread0.203 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations32
Published2009
Admission routes1
Has abstractyes

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