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Record W2067638860 · doi:10.1080/1478643031000094749

Atomic mechanism of the Re and Ru strengthening effect on the γ-γ′ interface of Ni-based single-crystal superalloys: A first-principles study

2003· article· en· W2067638860 on OpenAlexafffund
K. Chen, L.R. Zhao, John S. Tse

Bibliographic record

VenueThe Philosophical Magazine A Journal of Theoretical Experimental and Applied Physics · 2003
Typearticle
Languageen
FieldEngineering
TopicHigh Temperature Alloys and Creep
Canadian institutionsNational Research Council CanadaSteacie Institute for Molecular Sciences
FundersMinistère de la Défense Nationale
KeywordsSuperalloyCluster (spacecraft)Atom (system on chip)Materials scienceAtomic orbitalMolecular orbitalSingle crystalCrystal (programming language)CrystallographyPopulationMulliken population analysisDensity functional theoryElectronComputational chemistryChemical physicsChemistryMetallurgyMoleculePhysicsComputer scienceAlloyQuantum mechanics

Abstract

fetched live from OpenAlex

A possible atomic mechanism underlying the Re- and Ru-induced strengthening effects on the n- n' interface in Ni-based single-crystal superalloys has been investigated using the DMol3 molecular orbital package based on density functional theory. The calculation of bonding properties has been performed on a cluster designed to model Re and Ru strengthening effects within the interface. The stronger Re(Ru)--Ni bonds are formed mainly as a result of (Re(Ru) d-(Ni d) hybridization, while the Ni--Ni bonding become weaker accompanying the Re(Ru) substitution. The vertical and horizontal bond orders for a local environmental cluster are proposed and developed for the description of the strengthening effect on the n- n' interface, with larger bond order values achieving better effect. Results show that both Re and Ru significantly strengthen the interface. It is also shown that the strengthening effect of Re is better than that of Ru, and this is explained in terms of the charge transfer of electrons between orbitals of Ru atom according to Mulliken population analysis. The calculation results provide a basis for understanding the atomic mechanism of Re- and Ru-induced n- n' interfacial strengthening.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.528
Threshold uncertainty score0.489

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.001
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.012
GPT teacher head0.228
Teacher spread0.216 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations27
Published2003
Admission routes2
Has abstractyes

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