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Record W2069488589 · doi:10.1039/c4sm01490a

Streaming potential and electroviscous effects in soft nanochannels: towards designing more efficient nanofluidic electrochemomechanical energy converters

2014· article· en· W2069488589 on OpenAlexaff
Sourayon Chanda, Shayandev Sinha, Siddhartha Das

Bibliographic record

VenueSoft Matter · 2014
Typearticle
Languageen
FieldEngineering
TopicNanopore and Nanochannel Transport Studies
Canadian institutionsUniversity of Alberta
Fundersnot available
KeywordsStreaming currentZeta potentialNanotechnologyDonnan potentialPotential energyElectrostaticsElectric potential energyNanofluidicsElectric potentialDimensionless quantityMaterials scienceSoft matterPoisson–Boltzmann equationChemical physicsChemistryMechanicsEnergy (signal processing)ElectrodeIonVoltageNanoparticleClassical mechanicsElectrokinetic phenomenaPhysicsColloidPhysical chemistry

Abstract

fetched live from OpenAlex

In this paper we provide analytical solutions for the streaming potential and electroviscous effects in soft nanochannels. The analysis is based on the solution of the linearized Poisson-Boltzmann equation, valid for small electrostatic potentials. We identify the important dimensionless parameters that dictate these two effects. Results are provided for a large range of electric double layer (EDL) thickness values, spanning from the case of very thin to very large overlapped EDL thicknesses. We compare the results with those of a rigid nanochannel, having zeta potential equal to the electrostatic potential at the solid-polyelectrolyte interface of the soft nanochannels. For the soft nanochannel, the streaming potential varies very weakly with the EDL thickness and can be substantially larger than that corresponding to the rigid nanochannel. The electroviscous effects for the soft nanochannel, unlike the rigid nanochannel, virtually always exhibit a monotonic decrease with the EDL thickness, and for certain parameter ranges can be several times larger than that for a rigid nanochannel. Most importantly, for the soft nanochannels the electrochemomechanical energy conversion, associated with the generation of streaming potential, is found to be highly efficient, with the efficiency being several times higher than that of a rigid nanochannel.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.001
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Simulation or modeling · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.003

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.001
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.001
Scholarly communication0.0010.001
Open science0.0000.001
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.003
GPT teacher head0.175
Teacher spread0.172 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designSimulation or modeling
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations155
Published2014
Admission routes1
Has abstractyes

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