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Record W2071833140 · doi:10.1021/ma0102722

Photoinduced Birefringence and Surface Relief Gratings in Novel Polyurethanes with Azobenzene Groups in the Main Chain

2001· article· en· W2071833140 on OpenAlex
Yiliang Wu, Almeria Natansohn, P. Rochon

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.

Bibliographic record

VenueMacromolecules · 2001
Typearticle
Languageen
FieldMaterials Science
TopicLiquid Crystal Research Advancements
Canadian institutionsRoyal Military College of CanadaQueen's University
Fundersnot available
KeywordsBirefringenceAzobenzenePolymerMaterials scienceDiffractionIrradiationPolymer chemistryOpticsComposite material

Abstract

fetched live from OpenAlex

Three novel polyurethanes with V-shaped bisazo groups ( PU1 and PU2 ) or rodlike monoazo groups ( PU3 ) in the main chain were synthesized. On irradiation with a linearly polarized laser beam, birefringence was induced in the three films to the level of 0.035, 0.037, and 0.044 for PU1, PU2, and PU3, respectively. The stable birefringence obtained at T g − T = 33 °C was 71%, 46%, and 19% of that achieved at room temperature for PU1, PU2, and PU3, respectively. The relative stability of the photoinduced birefringence of PU3 decreased linearly with the increase of temperature, while that of PU1 and PU2 was constant even close to T g . Surface relief gratings with high diffraction efficiency were inscribed on these main-chain polymers. The photoinduced gratings are only partially erasable by heating above the T g of the polymers.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.032
Threshold uncertainty score0.559

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.001
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.018
GPT teacher head0.266
Teacher spread0.248 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it