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Record W2079425730 · doi:10.1021/jf2034237

Chemoenzymatic Synthesis of Phytosteryl Ferulates and Evaluation of Their Antioxidant Activity

2011· article· en· W2079425730 on OpenAlexaff
Zhuliang Tan, Fereidoon Shahidi

Bibliographic record

VenueJournal of Agricultural and Food Chemistry · 2011
Typearticle
Languageen
FieldMedicine
TopicCholesterol and Lipid Metabolism
Canadian institutionsMemorial University of Newfoundland
Fundersnot available
KeywordsAtmospheric-pressure chemical ionizationChemistryMass spectrometryCandida rugosaAntioxidantHigh-performance liquid chromatographyChromatographyFourier transform infrared spectroscopySelected ion monitoringOrganic chemistryChemical ionizationGas chromatography–mass spectrometryEnzymeIonizationLipaseIon

Abstract

fetched live from OpenAlex

The feasibility of a two-step chemoenzymatic synthesis of phytosteryl ferulates was successfully established in this work. An intermediate vinyl ferulate was first chemically produced and subsequently esterified with phytosterols through alcoholysis with Candida rugosa as a catalyst. The structures of phytosteryl ferulates were confirmed by Fourier transform infrared (FTIR) and high-performance chromatography-mass spectrometry/mass spectrometry (HPLC-MS/MS) using atmospheric pressure chemical ionization (APCI) under both positive and negative ion modes. The antioxidant activity of phytosteryl ferulates was higher than that of the starting material and the intermediate in the assays employed. The results indicated that phytosteryl ferulates had a good potential to be used as food antioxidants and may also serve as cholesterol-lowering agents.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.452
Threshold uncertainty score0.201

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.031
GPT teacher head0.233
Teacher spread0.202 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations63
Published2011
Admission routes1
Has abstractyes

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