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Record W2088269856 · doi:10.1063/1.2372316

Kinetics of the photostructural changes in a-Se films

2006· article· en· W2088269856 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.

Bibliographic record

VenueJournal of Applied Physics · 2006
Typearticle
Languageen
FieldMaterials Science
TopicPhase-change materials and chalcogenides
Canadian institutionsUniversity of SaskatchewanHealth Sciences CentreSunnybrook Health Science Centre
FundersDeutsche ForschungsgemeinschaftFonds der Chemischen IndustrieSusan G. Komen
KeywordsPhotodarkeningMetastabilityAmorphous solidStretched exponential functionKineticsMaterials scienceRelaxation (psychology)Activation energyCondensed matter physicsChemistryCrystallographyOptoelectronicsPhysical chemistryExponential functionPhysics

Abstract

fetched live from OpenAlex

The kinetics of the photodarkening effect has been studied experimentally for amorphous selenium (a-Se) layers at room temperature and at an elevated temperature (35°C) close to the glass transition. By switching an intense pumping light on and off with a period of 100s, we have studied the kinetics of both the buildup of photodarkening and its relaxation (recovery). It was found that at 35°C, only a reversible component of photodarkening has been observed. This result has been interpreted within the framework of a phenomenological model assuming that photodarkening is caused by light-induced transitions of structural units from their ground states into metastable states. Our estimate for the energy barrier EB between these states obtained for the photodarkening process (EB∼0.8eV) coincides with that obtained from the analysis of the relaxation process. At room temperature, an irreversible component of photodarkening has been observed along with the reversible one. The energy barrier responsible for the relaxation of the reversible component at room temperature appears the same as at 35°C. This suggests that the energy barrier identified represents a fundamental feature of the photoinduced structural metastability in amorphous selenium.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.010
Threshold uncertainty score0.269

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.018
GPT teacher head0.236
Teacher spread0.218 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it