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Record W2090669166 · doi:10.1021/ef049729+

Kinetics of Structure H Gas Hydrate

2005· article· en· W2090669166 on OpenAlexafffund
Ju Dong Lee, Robin Susilo, Peter Englezos

Bibliographic record

VenueEnergy & Fuels · 2005
Typearticle
Languageen
FieldEnvironmental Science
TopicMethane Hydrates and Related Phenomena
Canadian institutionsUniversity of British Columbia
FundersNatural Sciences and Engineering Research Council of Canada
KeywordsClathrate hydrateKineticsHydrateChemistryChemical engineeringMaterials scienceMineralogyOrganic chemistryPhysicsEngineering

Abstract

fetched live from OpenAlex

Experimental data on the kinetics of formation of structure H gas hydrate obtained in a semibatch stirred vessel at pressures of 0.63−1.5 MPa above equilibrium are reported. Methane was used as a guest substance and neohexane, tert -butyl methyl ether, and methylcyclohexane were used as the large molecule guest substance (LMGS). The results indicate that the rates of hydrate formation and the induction times are dependent on the magnitude of the driving force and the type of LMGS. When tert -butyl methyl ether is used as the LMGS, rapid hydrate formation and a much smaller induction time can be achieved. Furthermore, the methane consumption rate for hydrate formation in the presence of tert -butyl methyl ether is 3 times greater than that for a pure methane−water system. It was also observed that, although the induction period was greatly shortened by the memory effect, the rate of gas consumption rate was not affected. Hydrate decompositions were also conducted at a pressure 20% below equilibrium. The system with tert -butyl methyl ether as LMGS exhibited the fastest decomposition rate.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesInsufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.165
Threshold uncertainty score0.992

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0090.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.005
GPT teacher head0.195
Teacher spread0.190 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations100
Published2005
Admission routes2
Has abstractyes

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