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Record W2092547555 · doi:10.1021/jp4073729

Facile and Mild Strategy Toward Biopolymer-Coated Boron Nitride Nanotubes via a Glycine-Assisted Interfacial Process

2013· article· en· W2092547555 on OpenAlexaff
Yiu‐Ting R. Lau, Maho Yamaguchi, Xia Li, Yoshio Bando, Dmitri Golberg, Françoise M. Winnik

Bibliographic record

VenueThe Journal of Physical Chemistry C · 2013
Typearticle
Languageen
FieldMaterials Science
TopicElectrospun Nanofibers in Biomedical Applications
Canadian institutionsUniversité de MontréalUniversité du Québec à Montréal
FundersNational Institute for Materials Science
KeywordsBiopolymerPolymerChemical engineeringMaterials scienceBoron nitrideAqueous solutionAdsorptionSolventIonic bondingChitosanChemistryNanotechnologyOrganic chemistry

Abstract

fetched live from OpenAlex

We report a simple way to obtain polymer-coated multiwalled boron nitride nanotubes (BNNTs) conducted under mild conditions compatible with fragile biopolymers. The approach converts aggregated pristine BNNTs into colloidally stable dispersions in water without requiring treatment at high temperature or in strongly oxidative conditions. The method relies on our experimental observation that glycine (NH 2 –CH 2 –COOH, Gly) interacts with BNNTs, in accordance with theoretical calculations. The role of glycine in this process is 2-fold: the Gly amine group binds to the B-sites of BNNTs, while the Gly carboxylic acid function provides ionic anchoring sites for interactions with polyelectrolytes. The formation of Gly-BNNTs proved to be essential, since they readily disperse in water as disentangled objects and spontaneously adsorb polycations, such as chitosan (CH), polyanions, such as hyaluronan (HA), and polyzwitterionic polymers, such as chitosan-phosphorylcholine (CH-PC). Treatment of aqueous dispersions of coarsely coated BNNTs with an immiscible solvent (hexane) resulted in the complete coverage of the BNNT surfaces via oil/water interfacial assembly. This work provides a rapid, mild, and scalable route to water-dispersible biofunctional BNNTs that may serve as drug delivery vehicles or scaffolds in tissue engineering.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.002

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.012
GPT teacher head0.262
Teacher spread0.250 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations25
Published2013
Admission routes1
Has abstractyes

Explore more

Same venueThe Journal of Physical Chemistry CSame topicElectrospun Nanofibers in Biomedical ApplicationsFrench-language works237,207