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Record W2094687749 · doi:10.1021/ie060511f

Mechanical Properties of Polyelectrolyte Complex Films Based on Polyvinylamine and Carboxymethyl Cellulose

2006· article· en· W2094687749 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.

Bibliographic record

VenueIndustrial & Engineering Chemistry Research · 2006
Typearticle
Languageen
FieldMaterials Science
TopicPolymer Surface Interaction Studies
Canadian institutionsMcMaster University
Fundersnot available
KeywordsCarboxymethyl cellulosePolyelectrolyteUltimate tensile strengthIonic strengthAqueous solutionChemical engineeringPolymer chemistryPolymerCopolymerMaterials scienceChemistryHydrogen bondCelluloseComposite materialMoleculeOrganic chemistrySodium

Abstract

fetched live from OpenAlex

Homogeneous polyelectrolyte complex films were cast from mixtures of poly(vinylamine- co -vinylformamide) and carboxymethyl cellulose (CMC) in 50% formic acid aqueous solution with compositions varying between CMC blended with pure polyvinylamine (PVAm) and CMC blended with pure poly( N -vinylformamide) (PNVF). The tensile strength and tensile modulus of the complex films were measured as functions of polymer ratio, molecular weight, function group content, and water content. PVAm addition lowered the strength and modulus of dry CMC whereas PNVF did not; intermediate PVAm−PNVF copolymers gave intermediate results. Mechanical strength decreased with increasing molecular weight of CMC and carboxyl content, but was not affected by molecular weight of PVAm. The mechanical properties of all the films decreased with increasing water content. CMC:PVAm films were swollen gels in water, whereas CMC:PNVF films dissolved in water. Heating did not improve the mechanical strength, whereas cross-linking with 5% glutaraldehyde doubled the strength. It was proposed that hydrogen bonding was the predominant intermolecular force responsible for the strength of dry film blends whereas ionic bonds between CMC-carboxyl and PVAm-ammonium ions were responsible for the integrity of water swollen polyelectrolyte films.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.001
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.015
Threshold uncertainty score0.763

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.001
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.095
GPT teacher head0.306
Teacher spread0.211 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it