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Record W2101613836 · doi:10.1002/rcm.7246

High‐performance thin‐layer chromatography/desorption electrospray ionization mass spectrometry imaging of the crude extract from the peels of <i>Citrus aurantium</i> L. ( <i>Rutaceae</i> )

2015· article· en· W2101613836 on OpenAlexafffund
Bianca Souza Bagatela, Andrey Pereira Lopes, Elaine C. Cabral, Fábio Ferreira Perazzo, Demian R. Ifa

Bibliographic record

VenueRapid Communications in Mass Spectrometry · 2015
Typearticle
Languageen
FieldBiochemistry, Genetics and Molecular Biology
TopicMetabolomics and Mass Spectrometry Studies
Canadian institutionsIONICS Mass Spectrometry (Canada)York University
FundersNatural Sciences and Engineering Research Council of CanadaConselho Nacional de Desenvolvimento Científico e Tecnológico
KeywordsChemistryChromatographyMass spectrometryElectrospray ionizationRutaceaeElectrosprayTandem mass spectrometryMass spectrumDesorption electrospray ionizationIonizationChemical ionizationIonOrganic chemistry

Abstract

fetched live from OpenAlex

RATIONALE: Citrus aurantium L. is a plant belonging to the Rutaceae family, whose extracts are extensively used in weight management products and as thermogenic agents. Here we present two methodologies to analyse the extracts obtained from the peels of Citrus aurantium L. that usually require multiple sample preparation and detection steps. METHODS: Polar compounds of the crude extract from the peels of Citrus aurantium L. (Rutaceae) were investigated by direct infusion electrospray ionization mass spectrometry (ESI-MS) and high-performance thin-layer chromatography (HPTLC) coupled to desorption electrospray ionization mass spectrometry (DESI-MS). ESI-MS was performed in both positive and negative ion modes. Molecular imaging of the HPTLC plates was used for the direct analysis of the phytocompounds present in the crude extract from the peels of Citrus aurantium L. by DESI-MS imaging. RESULTS: Characteristic mass spectra with many diagnostic ions were obtained from the extract analysis, allowing a fast and reliable identification of these species. Tandem mass spectrometry (MS/MS) was employed to confirm the identity of specific metabolites. CONCLUSIONS: HPTLC/DESI-MS imaging is a relatively fast, versatile, and efficient technique for natural product analysis, since many more ions are observed than with the direct infusion ESI-MS. The MS/MS technique provided information about the component structures, revealing the presence of important bioactive components. The application of DESI-MS imaging may contribute to the improvement identification and characterization of pharmacologically active compounds in phytochemistry.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.051
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.003
Science and technology studies0.0000.001
Scholarly communication0.0000.000
Open science0.0020.001
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.016
GPT teacher head0.251
Teacher spread0.235 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations32
Published2015
Admission routes2
Has abstractyes

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