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Record W2107297909 · doi:10.1139/v03-056

Derivatives of tetraphenylmethane and tetraphenylsilane: Synthesis of new tetrahedral building blocks for molecular construction

2003· article· en· W2107297909 on OpenAlexvenueno aff
Jean‐Hugues Fournier, Xin Wang, James D. Wuest

Bibliographic record

VenueCanadian Journal of Chemistry · 2003
Typearticle
Languageen
FieldPharmacology, Toxicology and Pharmaceutics
TopicFluorine in Organic Chemistry
Canadian institutionsnot available
Fundersnot available
KeywordsSilaneChemistryHydroxymethylSupramolecular chemistryMethaneMoleculeTetrahedronOrganic chemistryPolymer chemistryCrystallography

Abstract

fetched live from OpenAlex

Useful derivatives of tetraphenylmethane and tetraphenylsilane have been synthesized by efficient methods that give crystalline products without chromatographic purification. New compounds include tetrakis(4-hydroxyphenyl)methane (21), tetrakis(4-formylphenyl)methane (22), tetrakis[(4-hydroxymethyl)phenyl]methane (23), tetrakis(4-bromophenyl)silane (24), tetrakis(4-iodophenyl)silane (25), tetrakis(4-hydroxyphenyl)silane (26), tetrakis[(4-hydroxymethyl)phenyl]silane (27), and tetrakis[(4-chloromethyl)phenyl]silane (28). These compounds are valuable precursors for the construction of complex molecules with tetrahedral geometries.Key words: organic synthesis, molecular and supramolecular design and construction, tetraphenylmethane, tetraphenyl silane, tetrahedral building blocks.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.002
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.015
Threshold uncertainty score0.906

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.002
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.035
GPT teacher head0.334
Teacher spread0.299 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations60
Published2003
Admission routes1
Has abstractyes

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