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Effect of Surface Fluorination on Diffusion through a High Density Polyethylene Geomembrane

2005· article· en· W2107904120 on OpenAlexaff
Henri P Sangam, R. Kerry Rowe

Bibliographic record

VenueJournal of Geotechnical and Geoenvironmental Engineering · 2005
Typearticle
Languageen
FieldEnvironmental Science
TopicLandfill Environmental Impact Studies
Canadian institutionsSNC-Lavalin (Canada)Queen's University
Fundersnot available
KeywordsGeomembraneHigh-density polyethylenePolyolefinLeachatePolyethyleneMaterials scienceSorptionPermeationDiffusionChemical engineeringGeotechnical engineeringComposite materialEnvironmental chemistryChemistryOrganic chemistryGeologyLayer (electronics)Adsorption

Abstract

fetched live from OpenAlex

The relative improvement of the diffusive barrier function of high density polyethylene (HDPE) geomembranes to volatile organic compounds (VOCs) when subjected to surface fluorination is experimentally examined. The surface fluorination consisted of applying elemental fluorine, which exchanged with hydrogen along polymer chains at the surface of a polyolefin substrate. Sorption and diffusion tests were performed on both traditional “untreated” and “fluorinated” 1.5mm HDPE geomembranes using dilute aqueous organic contaminants commonly found in municipal solid waste leachate. The partitioning coefficient is shown to remain essential the same after the surface fluorination; however, the surface fluorination resulted in a reduction in both the diffusion and the permeation coefficients by factors ranging between 1.5 and 4.5, depending on the hydrocarbon examined. Modeling of VOC diffusion through a geomembrane/compacted clay composite liner indicated that contaminant impacts were about 1.7–2.9 times lower when a fluorinated geomembrane is used. To achieve the same level of protection as provided by the fluorinated geomembrane underlain by 0.60m of compacted clay, one would need an additional 0.4–0.9m of compacted clay in conjunction with a conventional (untreated) geomembrane. The importance of the thickness of the treated layer is highlighted.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.001
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.002

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.001
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.002
GPT teacher head0.192
Teacher spread0.190 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations69
Published2005
Admission routes1
Has abstractyes

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