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Record W2110630633 · doi:10.1063/1.481549

High-resolution infrared spectrum and energy levels of the weakly bound complex, CO-orthoD2

2000· article· en· W2110630633 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.

Bibliographic record

VenueThe Journal of Chemical Physics · 2000
Typearticle
Languageen
FieldChemistry
TopicSpectroscopy and Laser Applications
Canadian institutionsSteacie Institute for Molecular Sciences
Fundersnot available
KeywordsChemistryInfraredAtomic physicsIntermolecular forceInfrared spectroscopyCarbon monoxideResolution (logic)MicrowaveRotational–vibrational spectroscopyAnalytical Chemistry (journal)Fourier transformMolecular physicsPhysicsOpticsMoleculeExcited state

Abstract

fetched live from OpenAlex

The infrared spectrum of the weakly bound complex CO-orthoD2, which accompanies the fundamental band of CO in the 4.7 μm region, has been recorded at high resolution using a long-path (≈200 m), low-temperature (≈47 K), absorption cell coupled either with a Fourier transform spectrometer or with a tunable infrared diode laser. A total of 275 transitions, constituting most (>85%) of the observed lines, have been rotationally assigned in terms of 83 discrete quantum states of the complex. The positions of most of these energy levels have been accurately determined (<0.001 cm−1) for both the vCO=0 and 1 vibrational states. The binding energy of the complex, relative to the zero-point level, was determined to be about 30 cm−1. Predicted microwave and millimeter wave frequencies are given for the pure rotational spectrum. The energy level pattern derived here, together with that determined previously for the analogous CO-paraH2 complex, provides direct and precise information for testing and refining the intermolecular potential energy surface of the carbon monoxide–hydrogen system.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.051
Threshold uncertainty score0.724

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.017
GPT teacher head0.254
Teacher spread0.237 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it