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Record W2111257128 · doi:10.1524/zpch.2008.6012

Power and Wavelength Dependence of Photoenhancement in (CdSe)ZnS-Dopamine in Aqueous Solution and Live Cells

2008· article· en· W2111257128 on OpenAlexafffund
Samuel Clarke, Sandeep T. Koshy, J. Zhang, Netta Cohen, Jay Nadeau

Bibliographic record

VenueZeitschrift für Physikalische Chemie · 2008
Typearticle
Languageen
FieldMaterials Science
TopicQuantum Dots Synthesis And Properties
Canadian institutionsMcGill University
FundersEngineering and Physical Sciences Research CouncilNatural Sciences and Engineering Research Council of Canada
KeywordsQuantum dotDopaminePhotoluminescenceAqueous solutionUltravioletWavelengthEndocytosisExcitationOptoelectronicsChemistryMaterials scienceIrradiationBiophysicsPhotochemistryNanotechnologyPhysicsPhysical chemistry

Abstract

fetched live from OpenAlex

CdSe(ZnS) quantum dots conjugated to the electron donor dopamine show enhancement of photoluminescence over a time course of seconds to minutes when exposed to ultraviolet or blue irradiation. This phenomenon is observed when the dots are in aqueous solution as well as after endocytosis by living cells. The rate of enhancement is directly related to the number of dopamine conjugates per quantum dot, and can be semi-quantitatively adjusted over a wide range. Uptake of the particles by cells is also dependent upon surface coverage, with moderate coverages proving ideal for both uptake and relative signal enhancement. The enhancement is strongly power-dependent and may also show dependence upon wavelength; however, direct excitation of the dopamine molecule is not necessary for the enhancement effect.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.004

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.016
GPT teacher head0.234
Teacher spread0.218 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations5
Published2008
Admission routes2
Has abstractyes

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