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Record W2113827433 · doi:10.5194/acp-10-8997-2010

Dynamic adjustment of climatological ozone boundary conditions for air-quality forecasts

2010· article· en· W2113827433 on OpenAlexaffabout
Paul A. Makar, Curtis Mooney, Jiangyi Zhang, Didier Davignon, M. Samaali, Michael D. Moran, Hao He, D. W. Tarasick, David Sills, Jack Chen

Bibliographic record

VenueAtmospheric chemistry and physics · 2010
Typearticle
Languageen
FieldEarth and Planetary Sciences
TopicAtmospheric Ozone and Climate
Canadian institutionsTransCanada (Canada)Alberta Environment and Protected AreasEnvironment and Climate Change Canada
Fundersnot available
KeywordsTropospheric ozoneOzoneTropopauseTroposphereEnvironmental scienceExtrapolationAtmospheric sciencesClimatologyAir quality indexMeteorologyGeographyGeologyMathematicsStatistics

Abstract

fetched live from OpenAlex

Abstract. Ten different approaches for applying lateral and top climatological boundary conditions for ozone have been evaluated using the off-line regional air-quality model AURAMS, driven with meteorology provided by the GEM weather-forecast model. All ten approaches employ the same climatological ozone profiles, but differ in the manner in which they are applied, via the inclusion or exclusion of (i) a dynamic adjustment of the climatological ozone profile in response to the model-predicted tropopause height, (ii) a sponge zone for ozone on the model top, (iii) upward extrapolation of the climatological ozone profile, and (iv) different mass consistency corrections. The model performance for each approach was evaluated against North American surface ozone and ozonesonde observations from the BAQS-Met field study period in the summer of 2007. The original daily one-hour maximum surface ozone biases of about +15 ppbv were greatly reduced (halved) in some simulations using alternative methodologies. However, comparisons to ozonesonde observations showed that the reduction in surface ozone bias sometimes came at the cost of significant positive biases in ozone concentrations in the free troposphere and upper troposphere. The best overall performance throughout the troposphere was achieved using a methodology that included dynamic tropopause height adjustment, no sponge zone at the model top, extrapolation of ozone when required above the limit of the climatology, and no mass consistency corrections (global mass conservation was still enforced). The simulation using this model version had a one-hour daily maximum surface ozone bias of +8.6 ppbv, with small reductions in model correlation, and the best comparison to ozonesonde profiles. This recommended and original methodologies were compared for two further case studies: a high-resolution simulation of the BAQS-Met measurement intensive, and a study of the downwind region of the Canadian Rockies. Significant improvements were noted for the high resolution simulations during the BAQS-Met measurement intensive period, both in formal statistical comparisons and time series comparisons of events at surface stations. The tests for the downwind-Rockies region showed that the coupling between vertical transport associated with troposphere/stratosphere exchange, and that associated with boundary layer turbulent mixing, may contribute to ozone positive biases. The results may be unique to the modelling setup employed, but the results also highlight the importance of evaluating boundary condition and mass consistency/correction algorithms against three-dimensional datasets.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.003
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Simulation or modeling · Consensus signal: Simulation or modeling
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.027
Threshold uncertainty score0.054

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0010.003
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0010.001
Open science0.0010.001
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.012
GPT teacher head0.257
Teacher spread0.245 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designSimulation or modeling
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations50
Published2010
Admission routes2
Has abstractyes

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